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DOI | 10.1021/acs.est.8b06575 |
Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China | |
Huang, Jie1,2; Kang, Shichang3,9![]() ![]() | |
发表日期 | 2019 |
ISSN | 0013-936X |
EISSN | 1520-5851 |
卷号 | 53期号:12页码:6632-6639 |
英文摘要 | Cryoconite is a granular aggregate, comprised of both mineral and biological material, and known to accumulate atmospheric contaminants. In this study, cryoconite was sampled from seven high-elevation glaciers in Western China to investigate the spatial and altitudinal patterns of atmospheric mercury (Hg) accumulation in the cryoconite. The results show that total Hg (Hg-T) concentrations in cryoconite were significant with relatively higher Hg accumulation in the southern glaciers (66.0 +/- 29.3 ng g(-1)), monsoon-influenced regions, than those in the northern glaciers (42.5 +/- 20.7 ng g(-1)), westerlies-influenced regions. The altitudinal profile indicates that Hg-T concentrations in the northern glaciers decrease significantly with altitude, while those in the southern glaciers generally increase toward higher elevations. Unexpectedly high accumulation of methyl-Hg (MeHg) with an average of 1.0 +/- 0.4 ng g(-1) was also detected in the cryoconite samples, revealing the surface of cryoconite could act as a potential site for Hg methylation in alpine environments. Our preliminary estimate suggests a storage of similar to 34.3 +/- 17.4 and 0.65 +/- 0.28 kg of Hg-T and MeHg from a single year of formation process in the glacier cryoconite. Therefore, glacier cryoconite could play an important role in Hg storage and transformation, which may result in downstream effects on glacier-fed ecosystems under climate warming scenario. |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
来源期刊 | ENVIRONMENTAL SCIENCE & TECHNOLOGY
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/99207 |
作者单位 | 1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China; 2.Chinese Acad Sci, CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China; 3.Chinese Acad Sci, Northeast Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China; 4.Southwest Univ, Coll Resources & Environm, Chongqing 400715, Peoples R China; 5.Chinese Acad Sci, Inst Geochem, State Key Lab Ore Deposit Geochem, Guiyang 550002, Guizhou, Peoples R China; 6.Banaras Hindu Univ, Inst Environm & Sustainable Dev, Varanasi 221005, Uttar Pradesh, India; 7.Univ Manitoba, Ctr Earth Observat Sci, Winnipeg, MB R3T 2N2, Canada; 8.Univ Manitoba, Dept Environm & Geog, Winnipeg, MB R3T 2N2, Canada; 9.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Huang, Jie,Kang, Shichang,Ma, Ming,et al. Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China[J],2019,53(12):6632-6639. |
APA | Huang, Jie.,Kang, Shichang.,Ma, Ming.,Guo, Junming.,Cong, Zhiyuan.,...&Wang, Feiyue.(2019).Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,53(12),6632-6639. |
MLA | Huang, Jie,et al."Accumulation of Atmospheric Mercury in Glacier Cryoconite over Western China".ENVIRONMENTAL SCIENCE & TECHNOLOGY 53.12(2019):6632-6639. |
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