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DOI10.1016/j.ijhydene.2019.02.121
Process analysis of hydrogen production from biomass gasification in fluidized bed reactor with different separation systems
Marcantonio, Vera1; De Falco, Marcello2; Capocelli, Mauro2; Bocci, Enrico3; Colantoni, Andrea1; Villarini, Mauro1
发表日期2019
ISSN0360-3199
EISSN1879-3487
卷号44期号:21页码:10350-10360
英文摘要

Gasification is one of the most effective and studied methods for producing energy and fuels from biomass as different biomass feedstock can be handled, with the generation of syngas consisting of H-2, CO, and CH4, which can be used for several applications. In this study, the gasification of hazelnut shells (biomass) within a circulating bubbling fluidized bed gasifier was analyzed for the first time through a quasi-equilibrium approach developed in the Aspen Plus environment and used to validate and improve an existing bubbling fluidized bed gasifier model. The gasification unit was integrated with a water-gas shift (WGS) reactor to increase the hydrogen content in the outlet stream and with a pressure swing adsorption (PSA) unit for hydrogen separation. The amount of dry H-2 obtained out of the gasifier was 31.3 mol%, and this value increased to 47.5 mol% after the WGS reaction. The simulation results were compared and validated against experimental data reported in the literature. The process model was then modified by replacing the PSA unit with a palladium membrane separation module. The final results of the present work allowed comparison of the effects of the two conditioning systems, PSA and palladium membrane, indicating a comparative increase in the hydrogen recovery ratio of 28.9% with the palladium membrane relative to the PSA configuration. (C) 2019 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.


WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels
来源期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/96627
作者单位1.Tuscia Univ Viterbo, Dept Agr & Forestry Sci DAFNE, Via San Camillo de Lellis Snc, I-01100 Viterbo, Italy;
2.Univ Campus Bio Medico Roma, Dept Engn, Unit Proc Engn, Via Alvaro del Portillo 21, I-00128 Rome, Italy;
3.Marconi Univ, Dept Nucl Subnucl & Radiat Phys, I-00193 Rome, Italy
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GB/T 7714
Marcantonio, Vera,De Falco, Marcello,Capocelli, Mauro,et al. Process analysis of hydrogen production from biomass gasification in fluidized bed reactor with different separation systems[J],2019,44(21):10350-10360.
APA Marcantonio, Vera,De Falco, Marcello,Capocelli, Mauro,Bocci, Enrico,Colantoni, Andrea,&Villarini, Mauro.(2019).Process analysis of hydrogen production from biomass gasification in fluidized bed reactor with different separation systems.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,44(21),10350-10360.
MLA Marcantonio, Vera,et al."Process analysis of hydrogen production from biomass gasification in fluidized bed reactor with different separation systems".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 44.21(2019):10350-10360.
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