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DOI | 10.1016/j.petrol.2018.12.034 |
CO2/N-2 mixture sequestration in depleted natural gas hydrate reservoirs | |
Zhou, Hang; Chen, Bingbing; Wang, Shenglong; Yang, Mingjun | |
发表日期 | 2019 |
ISSN | 0920-4105 |
EISSN | 1873-4715 |
卷号 | 175页码:72-82 |
英文摘要 | Carbon dioxide (CO2) emission is one of the primary causes of global warming, while CO2 storage is an effective way to solve this problem. Moreover, CO2 storage as CO2 hydrate is regarded as a viable and promising way. The development of natural gas hydrate mining technologies has provided a safe and appropriate method to store CO2 in depleted gas hydrate reservoirs. In addition, different concentrations of N-2 are contained in the captured CO2 from flue gas. Therefore, CO2 storage with different N-2 concentrations in depleted natural gas hydrate reservoirs with excess water was investigated in this study. Three types of gas (pure CO2, 90 mol%CO2 + 10 mol %N-2 and 80 mol%CO2 + 20 mol%N-2) and three pressures (3.0 MPa, 3.2 MPa and 3.5 MPa) in the constant pressure process were investigated. Magnetic Resonance Imaging (MRI) was employed to monitor the entire experimental process. The experimental results showed that the hydrate was nucleated and generated in different areas independently during the storage process. N-2 was beneficial for quick hydrate formation; however, pure CO2 was most efficient for hydrate formation from a long-term perspective. In addition, CO2 was primarily stored as hydrate; a portion of CO2 was stored in the form of gas; and a small amount of CO2 was dissolved in the pore water. Moreover, the CO2 storage density (226.56 kg/m(3)) was the highest at the conditions of 275.15 K and 3.5 MPa using 90 mol%CO2 + 10 mol%N-2 in the experiments. The highest CO2 storage density (229.99 kg/m(3)) calculated through water conversion occurred at the conditions of 275.15 K and 3.5 MPa using pure CO2. |
WOS研究方向 | Energy & Fuels ; Engineering |
来源期刊 | JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/95586 |
作者单位 | Dalian Univ Technol, Minist Educ, Key Lab Ocean Energy Utilizat & Energy Conservat, Dalian 116024, Liaoning, Peoples R China |
推荐引用方式 GB/T 7714 | Zhou, Hang,Chen, Bingbing,Wang, Shenglong,et al. CO2/N-2 mixture sequestration in depleted natural gas hydrate reservoirs[J],2019,175:72-82. |
APA | Zhou, Hang,Chen, Bingbing,Wang, Shenglong,&Yang, Mingjun.(2019).CO2/N-2 mixture sequestration in depleted natural gas hydrate reservoirs.JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING,175,72-82. |
MLA | Zhou, Hang,et al."CO2/N-2 mixture sequestration in depleted natural gas hydrate reservoirs".JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING 175(2019):72-82. |
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