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DOI10.1080/15567036.2018.1520331
The process intensification of CO2 absorption in Hilbert fractal reactor fabricated by a 3D printer
Zhang, Suqi1,2; Lu, Yue1,2; Sun, Jian1; Gu, Yu2; Zhang, Xiaodan2; Tang, Zhiyong2,3
发表日期2019
ISSN1556-7036
EISSN1556-7230
卷号41期号:4页码:481-492
英文摘要

CO2, as a major greenhouse gas, contributes greatly to the global warming. Increasing the efficiency of CO2 capture and utilization has becomea worldwide challenge. In the present research, Hilbert fractal reactor was fabricated via 3D printing technology for process intensification of ethanolamine (MEA) CO2 absorption. The performance of the Hilbert fractal reactor was investigated and compared to the serpentine reactor. For constant gas and liquid flow rates, the CO2 removal efficiency, the absorption rate, and the assumption of MEA increased with increasing concentration of MEA. In the comparison with the serpentine reactor, the CO2 removal efficiency in Hilbert fractal reactor is higher than that in the serpentine reactor at the relative low gas flow rate. The continuous bending in the Hilbert fractal reactor enhances the shear stress of the fluids, and the gas phase is segregated into the small bubbles which significantly increase the interface mass transfer. Under the relative high gas flow rate, the residence time of CO2 is short and the flow pattern in Hilbert reactor turns into the annular flow which adverse to CO2 absorption rate, and the advantage of Hilbert fractal reactor over serpentine reactor becomes negligible. The maximum CO2 removal efficiency of 57% was obtained in Hilbert fractal reactor.


WOS研究方向Energy & Fuels ; Engineering ; Environmental Sciences & Ecology
来源期刊ENERGY SOURCES PART A-RECOVERY UTILIZATION AND ENVIRONMENTAL EFFECTS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/93545
作者单位1.Shanghai Univ, Coll Environm & Chem Engn, Shanghai, Peoples R China;
2.Chinese Acad Sci, SARI, CAS Key Lab Low Carbon Convers Sci & Engn, Shanghai 201210, Peoples R China;
3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai, Peoples R China
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GB/T 7714
Zhang, Suqi,Lu, Yue,Sun, Jian,et al. The process intensification of CO2 absorption in Hilbert fractal reactor fabricated by a 3D printer[J],2019,41(4):481-492.
APA Zhang, Suqi,Lu, Yue,Sun, Jian,Gu, Yu,Zhang, Xiaodan,&Tang, Zhiyong.(2019).The process intensification of CO2 absorption in Hilbert fractal reactor fabricated by a 3D printer.ENERGY SOURCES PART A-RECOVERY UTILIZATION AND ENVIRONMENTAL EFFECTS,41(4),481-492.
MLA Zhang, Suqi,et al."The process intensification of CO2 absorption in Hilbert fractal reactor fabricated by a 3D printer".ENERGY SOURCES PART A-RECOVERY UTILIZATION AND ENVIRONMENTAL EFFECTS 41.4(2019):481-492.
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