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DOI10.1016/j.atmosenv.2018.11.028
Global changes in the diurnal cycle of surface ozone
Strode, Sarah A.1,2; Ziemke, Jerald R.2,3; Oman, Luke D.2; Lamsal, Lok N.1,2; Olsen, Mark A.2,3; Liu, Junhua1,2
发表日期2019
ISSN1352-2310
EISSN1873-2844
卷号199页码:323-333
英文摘要

Changing emissions of NOx and other ozone precursors drive trends in both production and loss of surface ozone, leading to surface ozone trends that differ according to the time of day. Consequently, the magnitude of the diurnal cycle in surface ozone is changing in several regions of the world. Changes in the diurnal cycle of ozone have implications for the metrics used to assess the impact of ozone on human health and vegetation, since different metrics are sensitive to different portions of the diurnal cycle. We use a high resolution model simulation to examine global changes in the magnitude of the diurnal cycle of O-3 between 1980 and 2015. The simulation reproduces the negative trends in the tropospheric NO2 column over the eastern United States and Europe, and the positive trends over East Asia, seen by the Ozone Monitoring Instrument (OMI). It also gives a reasonable reproduction of the change in the diurnal cycle of surface ozone seen at rural sites in the eastern United States between the 1990s and 2000s. The simulation shows that the magnitude of the surface O-3 diurnal cycle is increasing in regions with positive changes in NOx emissions, such as South and East Asia, and decreasing in regions with reductions in NOx emissions. It also shows changes in the diurnal cycle of the tropospheric ozone column, although these have fewer regions with statistically significant trends. These changes suggest that daily mean ozone is responding less than the mid-day ozone measured by the Total Ozone Mapping Spectrometer (TOMS) and OMI.


WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源期刊ATMOSPHERIC ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/93428
作者单位1.Univ Space Res Assoc, Columbia, MD USA;
2.NASA, Goddard Space Flight Ctr, Greenbelt, MD USA;
3.Morgan State Univ, Baltimore, MD 21239 USA
推荐引用方式
GB/T 7714
Strode, Sarah A.,Ziemke, Jerald R.,Oman, Luke D.,et al. Global changes in the diurnal cycle of surface ozone[J],2019,199:323-333.
APA Strode, Sarah A.,Ziemke, Jerald R.,Oman, Luke D.,Lamsal, Lok N.,Olsen, Mark A.,&Liu, Junhua.(2019).Global changes in the diurnal cycle of surface ozone.ATMOSPHERIC ENVIRONMENT,199,323-333.
MLA Strode, Sarah A.,et al."Global changes in the diurnal cycle of surface ozone".ATMOSPHERIC ENVIRONMENT 199(2019):323-333.
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