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DOI10.1016/j.scitotenv.2017.06.232
Deposition and light absorption characteristics of precipitation dissolved organic carbon (DOC) at three remote stations in the Himalayas and Tibetan Plateau, China
Li, Chaoliu1,3,4; Yan, Fangping3; Kang, Shichang2,4,5; Chen, Pengfei2; Hu, Zhaofu2,5; Han, Xiaowen1,5; Zhang, Guoshuai1; Gao, Shaopeng1; Qu, Bin3; Sillanpaa, Mika3,6
发表日期2017
ISSN0048-9697
EISSN1879-1026
卷号605页码:1039-1046
英文摘要

The concentrations, depositions and optical properties of precipitation DOC at three remote stations (Nam Co, Lulang and Everest) were investigated in the Himalayas and Tibetan Plateau (HTP). The results showed that their volume-weighted mean DOC concentrations were 1.05 +/- 1.01 mg C L-1, 0.83 +/- 0.85 mg C L-1 and 0.86 +/- 0.91mg C L-1, respectively, close to those of other remote areas in the world and lower than those of typical polluted urban cities. Combined with precipitation amounts, the DOC depositions at these three stations were calculated to be 0.34 +/- 0.32 g Cm-2 yr(-1), 0.84 +/- 0.86 g Cm-2 yr(-1) and 0.16 +/- 0.17 g Cm-2 yr(-1), respectively. The annual DOC deposition in the HTP was approximately 0.94 +/- 0.87 Tg C, the highest and lowest values appeared in the southeastern and northwestern plateau, respectively. The sources of DOC in the precipitation at these three stations were remarkably different, indicating large spatial heterogeneity in the sources of precipitation DOC over the HTP. Nam Co presented combustion sources from South Asia and local residents, Lulang showed biomass combustion source from South Asia, and Everest was mainly influenced by local mineral dust. The values of the MACDOC at 365 nm were 0.48 +/- 0.47 m(2) g(-1), 0.25 +/- 0.15 m(2) g(-1), and 0.64 +/- 0.49 m(2) g(-1), respectively, for the precipitation at the three stations. All of these values were significantly lower than those of corresponding near-surface aerosol samples because precipitation DOC contains more secondary organic aerosol with low light absorption abilities. Additionally, this phenomenon was also observed in seriously polluted urban areas, implying it is universal in the atmosphere. Because precipitation DOC contains information for both particle-bound and gaseous components from the near surface up to the altitude of clouds where precipitation occurs, the MAC(DOC) of precipitation is more representative than that of near-surface aerosols for a given region. (C) 2017 Elsevier B.V. All rights reserved.


英文关键词Dissolved organic carbon;The Third Pole;Deposition;Light absorption
语种英语
WOS研究方向Environmental Sciences & Ecology
来源期刊SCIENCE OF THE TOTAL ENVIRONMENT
来源机构中国科学院西北资源环境生态研究院
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/89618
作者单位1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China;;
2.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China;;
3.Lappeenranta Univ Technol, Lab Green Chem, Sammonkatu 12, Mikkeli 50130, Finland;;
4.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China;;
5.Univ Chinese Acad Sci, Beijing 100049, Peoples R China;;
6.Florida Int Univ, Dept Civil & Environm Engn, Miami, FL 33174 USA
推荐引用方式
GB/T 7714
Li, Chaoliu,Yan, Fangping,Kang, Shichang,et al. Deposition and light absorption characteristics of precipitation dissolved organic carbon (DOC) at three remote stations in the Himalayas and Tibetan Plateau, China[J]. 中国科学院西北资源环境生态研究院,2017,605:1039-1046.
APA Li, Chaoliu.,Yan, Fangping.,Kang, Shichang.,Chen, Pengfei.,Hu, Zhaofu.,...&Sillanpaa, Mika.(2017).Deposition and light absorption characteristics of precipitation dissolved organic carbon (DOC) at three remote stations in the Himalayas and Tibetan Plateau, China.SCIENCE OF THE TOTAL ENVIRONMENT,605,1039-1046.
MLA Li, Chaoliu,et al."Deposition and light absorption characteristics of precipitation dissolved organic carbon (DOC) at three remote stations in the Himalayas and Tibetan Plateau, China".SCIENCE OF THE TOTAL ENVIRONMENT 605(2017):1039-1046.
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