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DOI10.1016/j.scitotenv.2018.01.265
Dissolved organic carbon fractionation accelerates glacier-melting: A case study in the northern Tibetan Plateau
Hu, Zhaofu1,5; Kang, Shichang1,4,5; Yan, Fangping3; Zhang, Yulan1; Li, Yang2,3,5; Chen, Pengfei1; Qin, Xiang1; Wang, Kun1,5; Gao, Shaopeng2; Li, Chaoliu2,4
发表日期2018
ISSN0048-9697
EISSN1879-1026
卷号627页码:579-585
英文摘要

In glacierized regions, melting process has a significant effect on concentrations and light absorption characteristics of dissolved organic carbon (DOC), potentially resulting in variations of its radiative forcing, which is not yet relevant research at glacier region of the Tibetan Plateau (TP). In this study, DOC fractionation and its radiative forcing change during the melting process were investigated at Laohugou glacier No. 12 (LHG glacier) in western Qilian Mts., northern TP. DOC concentrations in fresh snow, snowpit and surface ice samples were 0.38 +/- 0.06, 0.22 +/- 0.11 and 0.60 +/- 0.21 mg L-1, respectively. Their mass absorption cross-section at 365 nm (MAC(365)) were 0.65 +/- 0.16, 4.71 +/- 3.68 and 1.44 +/- 0.52 m(2) g(-1), respectively. The MAC(365) values of snowpit samples showed a significant negative correlation with DOC concentrations, indicating DOC with high MAC(365) values were likely to be kept in snow during the melting process. Topsoil samples of LHG glacierized region likely contributed a lot to snowpit DOC with high MAC365 values due to their similar absorption spectra. Spatially, the DOC concentration of surface ice samples increased from terminus to the upper part of the glacier. Correspondingly, the MAC(365) value showed decreased trend. In the freezing experiment on surface ice and topsoil samples, small part of DOC with high MAC(365) value was also likely to enter first frozen solid phase. In addition, the radiative forcing caused by snowpit and surface ice DOC increased around 7.64 +/- 2.93 and 4.95 +/- 1.19 times relative to fresh snow DOC, indicating the snow/ice melting caused by increased light-absorbing DOC needs to be considered in the future research. (c) 2018 Elsevier B.V. All rights reserved.


英文关键词Melting process;Dissolved organic carbon;Concentration;Light absorption characteristic;The Tibetan Plateau
语种英语
WOS研究方向Environmental Sciences & Ecology
来源期刊SCIENCE OF THE TOTAL ENVIRONMENT
来源机构中国科学院西北资源环境生态研究院
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/89586
作者单位1.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Gansu, Peoples R China;;
2.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100085, Peoples R China;;
3.Lappeenranta Univ Technol, Lab Green Chem, Sammonkatu 12, Mikkeli 50130, Finland;;
4.Chinese Acad Sci, CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China;;
5.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
推荐引用方式
GB/T 7714
Hu, Zhaofu,Kang, Shichang,Yan, Fangping,et al. Dissolved organic carbon fractionation accelerates glacier-melting: A case study in the northern Tibetan Plateau[J]. 中国科学院西北资源环境生态研究院,2018,627:579-585.
APA Hu, Zhaofu.,Kang, Shichang.,Yan, Fangping.,Zhang, Yulan.,Li, Yang.,...&Li, Chaoliu.(2018).Dissolved organic carbon fractionation accelerates glacier-melting: A case study in the northern Tibetan Plateau.SCIENCE OF THE TOTAL ENVIRONMENT,627,579-585.
MLA Hu, Zhaofu,et al."Dissolved organic carbon fractionation accelerates glacier-melting: A case study in the northern Tibetan Plateau".SCIENCE OF THE TOTAL ENVIRONMENT 627(2018):579-585.
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