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DOI10.5194/acp-18-6441-2018
Seasonal variation and light absorption property of carbonaceous aerosol in a typical glacier region of the southeastern Tibetan Plateau
Niu H.;   Kang S.;   Wang H.;   Zhang R.;   Lu X.;   Qian Y.;   Paudyal R.;   Wang S.;   Shi X.;   Yan X.
发表日期2018
ISSN16807316
卷号18期号:9
英文摘要Deposition and accumulation of light-absorbing carbonaceous aerosol on glacier surfaces can alter the energy balance of glaciers. In this study, 2 years (December 2014 to December 2016) of continuous observations of carbonaceous aerosols in the glacierized region of the Mt. Yulong and Ganhaizi (GHZ) basin are analyzed. The average elemental carbon (EC) and organic carbon (OC) concentrations were 1.51±0.93 and 2.57±1.32 μmg-3, respectively. Although the annual mean OC EC ratio was 2.45±1.96, monthly mean EC concentrations during the post-monsoon season were even higher than OC in the high altitudes (approximately 5000 mga. s. l.) of Mt. Yulong. Strong photochemical reactions and local tourism activities were likely the main factors inducing high OC EC ratios in the Mt. Yulong region during the monsoon season. The mean mass absorption efficiency (MAE) of EC, measured for the first time in Mt. Yulong, at 632 nm with a thermal-optical carbon analyzer using the filter-based method, was 6.82±0.73 m2ggg-1, comparable with the results from other studies. Strong seasonal and spatial variations of EC MAE were largely related to the OC abundance. Source attribution analysis using a global aerosol-climate model, equipped with a black carbon (BC) source tagging technique, suggests that East Asia emissions, including local sources, have the dominant contribution (over 50 %) to annual mean near-surface BC in the Mt. Yulong area. There is also a strong seasonal variation in the regional source apportionment. South Asia has the largest contribution to near-surface BC during the pre-monsoon season, while East Asia dominates the monsoon season and post-monsoon season. Results in this study have great implications for accurately evaluating the influences of carbonaceous matter on glacial melting and water resource supply in glacierization areas. © 2018 Author(s).
URLhttps://www2.scopus.com/inward/record.uri?eid=2-s2.0-85046849352&doi=10.5194%2facp-18-6441-2018&partnerID=40&md5=495c0cf21351a0970b3916096d3753d6
语种英语
scopus关键词absorption; aerosol; atmospheric chemistry; concentration (composition); elemental carbon; energy balance; glacier; monsoon; organic carbon; seasonal variation; China; Qinghai-Xizang Plateau; Yulong Snow Mountains; Yunnan
来源期刊Atmospheric Chemistry and Physics
来源机构中国科学院西北生态环境资源研究院
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/77307
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GB/T 7714
Niu H.; Kang S.; Wang H.; Zhang R.; Lu X.; Qian Y.; Paudyal R.; Wang S.; Shi X.; Yan X.. Seasonal variation and light absorption property of carbonaceous aerosol in a typical glacier region of the southeastern Tibetan Plateau[J]. 中国科学院西北生态环境资源研究院,2018,18(9).
APA Niu H.; Kang S.; Wang H.; Zhang R.; Lu X.; Qian Y.; Paudyal R.; Wang S.; Shi X.; Yan X..(2018).Seasonal variation and light absorption property of carbonaceous aerosol in a typical glacier region of the southeastern Tibetan Plateau.Atmospheric Chemistry and Physics,18(9).
MLA Niu H.; Kang S.; Wang H.; Zhang R.; Lu X.; Qian Y.; Paudyal R.; Wang S.; Shi X.; Yan X.."Seasonal variation and light absorption property of carbonaceous aerosol in a typical glacier region of the southeastern Tibetan Plateau".Atmospheric Chemistry and Physics 18.9(2018).
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