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DOI | 10.1021/acs.est.7b05509 |
Sensitivity of Ambient Atmospheric Formaldehyde and Ozone to Precursor Species and Source Types Across the United States | |
Luecken, D. J.1; Napelenok, S. L.1; Strum, M.2; Scheffe, R.2; Phillips, S.2 | |
发表日期 | 2018-04-17 |
ISSN | 0013-936X |
卷号 | 52期号:8页码:4668-4675 |
英文摘要 | Formaldehyde (HCHO) is an important air pollutant from both an atmospheric chemistry and human health standpoint. This study uses an instrumented photochemical Air Quality Model, CMAQ-DDM, to identify the sensitivity of HCHO concentrations across the United States (U.S.) to major source types and hydrocarbon speciation. In July, biogenic sources of hydrocarbons contribute the most (92% of total hydrocarbon sensitivity), split between isoprene and other alkenes. Among anthropogenic sources, mobile sources of hydrocarbons and nitrogen oxides (NOx) dominate. In January, HCHO is more sensitive to anthropogenic hydrocarbons than biogenic sources, especially mobile sources and residential wood combustion (36% of national hydrocarbon sensitivity). While ozone (O-3) is three times more sensitive to NOx than hydrocarbons across most areas of the U.S., HCHO is six times more sensitive to hydrocarbons than NOx, largely due to sensitivity to biogenic precursors and the importance of low-NOx chemistry. In winter, both HCHO and O-3 show negative sensitivity to NOx (increases with the removal of NOx), although O-3 increases are larger. Relative sensitivities do not change substantially across different regions of the country. |
语种 | 英语 |
WOS记录号 | WOS:000430515400020 |
来源期刊 | ENVIRONMENTAL SCIENCE & TECHNOLOGY |
来源机构 | 美国环保署 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/62564 |
作者单位 | 1.US EPA, Off Res & Dev, Natl Exposure Res Lab, Res Triangle Pk, NC 27711 USA; 2.US EPA, Off Air Qual Planning & Stand, Res Triangle Pk, NC 27711 USA |
推荐引用方式 GB/T 7714 | Luecken, D. J.,Napelenok, S. L.,Strum, M.,et al. Sensitivity of Ambient Atmospheric Formaldehyde and Ozone to Precursor Species and Source Types Across the United States[J]. 美国环保署,2018,52(8):4668-4675. |
APA | Luecken, D. J.,Napelenok, S. L.,Strum, M.,Scheffe, R.,&Phillips, S..(2018).Sensitivity of Ambient Atmospheric Formaldehyde and Ozone to Precursor Species and Source Types Across the United States.ENVIRONMENTAL SCIENCE & TECHNOLOGY,52(8),4668-4675. |
MLA | Luecken, D. J.,et al."Sensitivity of Ambient Atmospheric Formaldehyde and Ozone to Precursor Species and Source Types Across the United States".ENVIRONMENTAL SCIENCE & TECHNOLOGY 52.8(2018):4668-4675. |
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