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DOI10.5194/acp-18-10199-2018
Modeled deposition of nitrogen and sulfur in Europe estimated by 14 air quality model systems: evaluation, effects of changes in emissions and implications for habitat protection
Vivanco, Marta G.1; Theobald, Mark R.1; Garcia-Gomez, Hector1; Luis Garrido, Juan1; Prank, Marje2,3; Aas, Wenche4; Adani, Mario5; Alyuz, Ummugulsum6; Andersson, Camilla7; Bellasio, Roberto8; Bessagnet, Bertrand9; Bianconi, Roberto8; Bieser, Johannes10; Brandt, Jurgen11; Briganti, Gino5; Cappelletti, Andrea5; Curci, Gabriele12; Christensen, Jesper H.11; Colette, Augustin9; Couvidat, Florian9; Cuvelier, Cornelis13; D'; Isidoro, Massimo5; Flemming, Johannes14; Fraser, Andrea15; Geels, Camilla11; Hansen, Kaj M.11; Hogrefe, Christian16; Im, Ulas11; Jorba, Oriol17; Kitwiroon, Nutthida18; Manders, Astrid19; Mircea, Mihaela5; Otero, Noelia20; Pay, Maria-Teresa17; Pozzoli, Luca21; Solazzo, Efisio21; Tsyro, Svetlana22; Unal, Alper23; Wind, Peter22,24; Galmarini, Stefano21
发表日期2018-07-17
ISSN1680-7316
卷号18期号:14页码:10199-10218
英文摘要

The evaluation and intercomparison of air quality models is key to reducing model errors and uncertainty. The projects AQMEII3 and EURODELTA-Trends, in the framework of the Task Force on Hemispheric Transport of Air Pollutants and the Task Force on Measurements and Modelling, respectively (both task forces under the UNECE Convention on the Long Range Transport of Air Pollution, LTRAP), have brought together various regional air quality models to analyze their performance in terms of air concentrations and wet deposition, as well as to address other specific objectives.


This paper jointly examines the results from both project communities by intercomparing and evaluating the deposition estimates of reduced and oxidized nitrogen (N) and sulfur (S) in Europe simulated by 14 air quality model systems for the year 2010. An accurate estimate of deposition is key to an accurate simulation of atmospheric concentrations. In addition, deposition fluxes are increasingly being used to estimate ecological impacts. It is therefore important to know by how much model results differ and how well they agree with observed values, at least when comparison with observations is possible, such as in the case of wet deposition.


This study reveals a large variability between the wet deposition estimates of the models, with some performing acceptably (according to previously defined criteria) and others underestimating wet deposition rates. For dry deposition, there are also considerable differences between the model estimates. An ensemble of the models with the best performance for N wet deposition was made and used to explore the implications of N deposition in the conservation of protected European habitats. Exceedances of empirical critical loads were calculated for the most common habitats at a resolution of 100 x 100m(2) within the Natura 2000 network, and the habitats with the largest areas showing exceedances are determined.


Moreover, simulations with reduced emissions in selected source areas indicated a fairly linear relationship between reductions in emissions and changes in the deposition rates of N and S. An approximate 20% reduction in N and S deposition in Europe is found when emissions at a global scale are reduced by the same amount. European emissions are by far the main contributor to deposition in Europe, whereas the reduction in deposition due to a decrease in emissions in North America is very small and confined to the western part of the domain. Reductions in European emissions led to substantial decreases in the protected habitat areas with critical load exceedances (halving the exceeded area for certain habitats), whereas no change was found, on average, when reducing North American emissions in terms of average values per habitat.


语种英语
WOS记录号WOS:000438945300005
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/62081
作者单位1.CIEMAT, Environm Dept, E-28040 Madrid, Spain;
2.Finnish Meteorol Inst, FI-00560 Helsinki, Finland;
3.Cornell Univ, Ithaca, NY 14850 USA;
4.NILU Norwegian Inst Air Res, N-2007 Kjeller, Norway;
5.Italian Natl Agcy New Technol Energy & Sustainabl, ENEA, Via Martini Monte Sole 4, I-40129 Bologna, Italy;
6.Bahcesehir Univ Engn & Nat Sci Fac, TR-34353 Besiktas, Turkey;
7.Swedish Meteorol & Hydrol Inst Norrkoping, SMHI, Norrkoping, Sweden;
8.Enviroware Srl, Concorezzo, MB, Italy;
9.Inst Natl Environm Ind & Risques, INERIS, Parc Alata, F-60550 Verneuil En Halatte, France;
10.Helmholtz Zentrum Geesthacht, Inst Coastal Res, Chem Transport Modelling Grp, Geesthacht, Germany;
11.Aarhus Univ, Dept Environm Sci, DK-4000 Roskilde, Denmark;
12.Univ Aquila, Dept Phys & Chem Sci, Laquila, Italy;
13.Ex European Commiss, Joint Res Ctr, I-21020 Ispra, Va, Italy;
14.European Ctr Medium Range Weather Forecasts, Reading, Berks, England;
15.Ricardo Energy & Environm, Gemini Bldg,Fermi Ave, Harwell OX11 0QR, Oxon, England;
16.US EPA, Computat Exposure Div, Natl Exposure Res Lab, Off Res & Dev, Res Triangle Pk, NC 27711 USA;
17.Barcelona Supercomp Ctr, Ctr Nacl Supercomp, Nexus 2 Bldg,Jordi Girona 29, Barcelona 08034, Spain;
18.Kings Coll London, Environm Res Grp, London, England;
19.Netherlands Org Appl Sci Res TNO, Utrecht, Netherlands;
20.Inst Adv Sustainabil Studies, Potsdam, Germany;
21.European Commiss, Joint Res Ctr, Ispra, VA, Italy;
22.Norwegian Meteorol Inst MET Norway, Res & Dev Dept, Climate Modelling & Air Pollut Div, POB 43, N-0313 Oslo, Norway;
23.Istanbul Tech Univ, Eurasia Inst Earth Sci, Istanbul, Turkey;
24.Univ Tromso, Fac Sci & Technol, Tromso, Norway
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Vivanco, Marta G.,Theobald, Mark R.,Garcia-Gomez, Hector,et al. Modeled deposition of nitrogen and sulfur in Europe estimated by 14 air quality model systems: evaluation, effects of changes in emissions and implications for habitat protection[J]. 美国环保署,2018,18(14):10199-10218.
APA Vivanco, Marta G..,Theobald, Mark R..,Garcia-Gomez, Hector.,Luis Garrido, Juan.,Prank, Marje.,...&Galmarini, Stefano.(2018).Modeled deposition of nitrogen and sulfur in Europe estimated by 14 air quality model systems: evaluation, effects of changes in emissions and implications for habitat protection.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(14),10199-10218.
MLA Vivanco, Marta G.,et al."Modeled deposition of nitrogen and sulfur in Europe estimated by 14 air quality model systems: evaluation, effects of changes in emissions and implications for habitat protection".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.14(2018):10199-10218.
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