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DOI10.1088/1748-9326/10/11/114014
Premature deaths attributed to source-specific BC emissions in six urban US regions
Turner, Matthew D.1; Henze, Daven K.1; Capps, Shannon L.1; Hakami, Amir2; Zhao, Shunliu2; Resler, Jaroslav3; Carmichael, Gregory R.4; Stanier, Charles O.4; Baek, Jaemeen4; Sandu, Adrian5; Russell, Armistead G.6; Nenes, Athanasios7; Pinder, Rob W.8; Napelenok, Sergey L.8; Bash, Jesse O.8; Percell, Peter B.9; Chai, Tianfeng10
发表日期2015-11-01
ISSN1748-9326
卷号10期号:11
英文摘要

Recent studies have shown that exposure to particulate black carbon (BC) has significant adverse health effects and may be more detrimental to human health than exposure to PM2.5 as a whole. Mobile source BC emission controls, mostly on diesel-burning vehicles, have successfully decreased mobile source BC emissions to less than half of what they were 30 years ago. Quantification of the benefits of previous emissions controls conveys the value of these regulatory actions and provides a method by which future control alternatives could be evaluated. In this study we use the adjoint of the Community Multiscale Air Quality (CMAQ) model to estimate highly-resolved spatial distributions of benefits related to emission reductions for six urban regions within the continental US. Emissions from outside each of the six chosen regions account for between 7% and 27% of the premature deaths attributed to exposure to BC within the region. While we estimate that nonroad mobile and onroad diesel emissions account for the largest number of premature deaths attributable to exposure to BC, onroad gasoline is shown to have more than double the benefit per unit emission relative to that of nonroad mobile and onroad diesel. Within the region encompassing New York City and Philadelphia, reductions in emissions from large industrial combustion sources that are not classified as EGUs (i.e., non-EGU) are estimated to have up to triple the benefits per unit emission relative to reductions to onroad diesel sectors, and provide similar benefits per unit emission to that of onroad gasoline emissions in the region. While onroad mobile emissions have been decreasing in the past 30 years and a majority of vehicle emission controls that regulate PM focus on diesel emissions, our analysis shows the most efficient target for stricter controls is actually onroad gasoline emissions.


英文关键词source attribution;particulate matter;aerosols;air quality;human well-being
语种英语
WOS记录号WOS:000367249900018
来源期刊ENVIRONMENTAL RESEARCH LETTERS
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/61837
作者单位1.Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA;
2.Carleton Univ, Dept Civil & Environm Engn, Ottawa, ON K1S 5B6, Canada;
3.Inst Comp Sci, Nonlinear Modeling, Prague 18207, Czech Republic;
4.Univ Iowa, Dept Chem & Biochem Engn, Iowa City, IA 52242 USA;
5.Virginia Tech, Comp Sci, Blacksburg, VA 24061 USA;
6.Georgia Tech, Sch Civil & Environm Engn, Atlanta, GA 30331 USA;
7.Georgia Tech, Sch Earth & Atmospher Sci, Atlanta, GA 30331 USA;
8.US EPA, Atmospher Modeling & Anal Div, Res Triangle Pk, NC 27711 USA;
9.Univ Houston, Dept Geosci, Houston, TX 77004 USA;
10.Univ Maryland, Coll Comp Math & Nat Sci, College Pk, MD 20742 USA
推荐引用方式
GB/T 7714
Turner, Matthew D.,Henze, Daven K.,Capps, Shannon L.,et al. Premature deaths attributed to source-specific BC emissions in six urban US regions[J]. 美国环保署,2015,10(11).
APA Turner, Matthew D..,Henze, Daven K..,Capps, Shannon L..,Hakami, Amir.,Zhao, Shunliu.,...&Chai, Tianfeng.(2015).Premature deaths attributed to source-specific BC emissions in six urban US regions.ENVIRONMENTAL RESEARCH LETTERS,10(11).
MLA Turner, Matthew D.,et al."Premature deaths attributed to source-specific BC emissions in six urban US regions".ENVIRONMENTAL RESEARCH LETTERS 10.11(2015).
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