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DOI10.1016/j.scitotenv.2017.03.262
Airborne measurements of isoprene and monoterpene emissions from southeastern US forests
Yu, Haofei1,2; Guenther, Alex2,3; Gu, Dasa2,3; Warneke, Carsten4,5; Geron, Chris6; Goldstein, Allen7; Graus, Martin8; Karl, Thomas8; Kaser, Lisa9; Misztal, Pawel7; Yuan, Bin4,5
发表日期2017-10-01
ISSN0048-9697
卷号595页码:149-158
英文摘要

Isoprene and monoterpene emission rates are essential inputs for atmospheric chemistry models that simulate atmospheric oxidant and particle distributions. Process studies of the biochemical and physiological mechanisms controlling these emissions are advancing our understanding and the accuracy of model predictions but efforts to quantify regional emissions have been limited by a lack of constraints on regional distributions of ecosystem emission capacities. We used an airborne wavelet-based eddy covariance measurement technique to characterize isoprene and monoterpene fluxes with high spatial resolution during the 2013 SAS (Southeast Atmosphere Study) in the southeastern United States. The fluxes measured by direct eddy covariance were comparable to emissions independently estimated using an indirect inverse modeling approach. Isoprene emission factors based on the aircraft wavelet flux estimates for high isoprene chemotypes (e.g., oaks) were similar to the MEGAN2.1 biogenic emission model estimates for landscapes dominated by oaks. Aircraft flux measurement estimates for landscapes with fewer isoprene emitting trees (e.g., pine plantations), were about a factor of two lower than MEGAN2.1 model estimates. The tendency for high isoprene emitters in these landscapes to occur in the shaded understory, where light dependent isoprene emissions are diminished, may explain the lower than expected emissions. This result demonstrates the importance of accurately representing the vertical profile of isoprene emitting biomass in biogenic emission models. Airborne measurement-based emission factors for high monoterpene chemotypes agreed with MEGAN2.1 in landscapes dominated by pine (high monoterpene chemotype) trees but were more than a factor of three higher than model estimates for landscapes dominated by oak (relatively low monoterpene emitting) trees. This results suggests that unaccounted processes, such as floral emissions or light dependent monoterpene emissions, or vegetation other than high monoterpene emitting trees may be an important source of monoterpene emissions in those landscapes and should be identified and included in biogenic emission models. (C) 2017 Elsevier B.V. All rights reserved.


英文关键词Isoprene;Monoterpenes;Biogenic volatile organic compounds;Aircraft flux measurements;Model of Emissions of Gases and Aerosols from;Nature (MEGAN)
语种英语
WOS记录号WOS:000401556800017
来源期刊SCIENCE OF THE TOTAL ENVIRONMENT
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/61801
作者单位1.Univ Cent Florida, Dept Civil Environm & Construct Engn, Orlando, FL 32816 USA;
2.Pacific Northwest Natl Lab, Richland, WA 99354 USA;
3.Univ Calif Irvine, Dept Earth Syst Sci, 3200 Croul Hall, Irvine, CA 92697 USA;
4.NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO USA;
5.Univ Colorado, CIRES, Boulder, CO 80309 USA;
6.US EPA, Natl Risk Management Res Lab, Raleigh, NC USA;
7.Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA;
8.Univ Innsbruck, Inst Atmospher & Cryospher Sci, Innsbruck, Austria;
9.Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA
推荐引用方式
GB/T 7714
Yu, Haofei,Guenther, Alex,Gu, Dasa,et al. Airborne measurements of isoprene and monoterpene emissions from southeastern US forests[J]. 美国环保署,2017,595:149-158.
APA Yu, Haofei.,Guenther, Alex.,Gu, Dasa.,Warneke, Carsten.,Geron, Chris.,...&Yuan, Bin.(2017).Airborne measurements of isoprene and monoterpene emissions from southeastern US forests.SCIENCE OF THE TOTAL ENVIRONMENT,595,149-158.
MLA Yu, Haofei,et al."Airborne measurements of isoprene and monoterpene emissions from southeastern US forests".SCIENCE OF THE TOTAL ENVIRONMENT 595(2017):149-158.
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