CCPortal
DOI10.1002/2017EF000588
Climate-driven exceedance of total (wet plus dry) nitrogen (N) plus sulfur (S) deposition to forest soil over the conterminous US
Sun, Jian1; Fu, Joshua S.1,2,3; Lynch, Jason A.4; Huang, Kan1,5; Gao, Yang6
发表日期2017-06-01
ISSN2328-4277
卷号5期号:6页码:560-576
英文摘要

Nitrogen (N) and sulfur (S) depositions are much mitigated over the conterminous U.S. (CONUS) but deposition exceedance still exists on forest soil. In addition, the empirical approach is usually used but only provides a spatially constant critical load (CL). Therefore, the CL derived from steady-state mass balance equation is used to study the CL exceedance on forest soil over the CONUS. The multimodel mean (MMM) of global climate-chemistry models in 2000s indicates that total (wet + dry) N deposition alone over 10.32% of forest soil exceeds the CL, but a higher percent (30.16%) is observed by the N + S deposition, which highlights the necessity of considering S deposition. In 2050s, less CL-exceeded forest soil is projected and the exceedance amount is lower as well, mainly attributed to the strong reduction of projected NOX and SO2 emissions. By first projecting the future CL due to the climate change, the CL exceedance could further decrease as the air temperature is projected to increase rapidly and lead to higher CL in the future. The CL exceedance by N deposition alone is likely to be dominated by NOy in 2000s but NHX in 2050s because of the enhanced NH3 emission. Moreover, both in 2000s and 2050s, using the CL generated by different aggregation methods can cause up to 33 times difference between the corresponding CL exceedance. This suggests that several regions are under the marginal threat of either N or N + S deposition and different CL can influence the results significantly.


语种英语
WOS记录号WOS:000405474400002
来源期刊EARTHS FUTURE
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/61297
作者单位1.Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA;
2.Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37830 USA;
3.Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37830 USA;
4.US EPA, Clean Air Markets Div, Washington, DC 20460 USA;
5.Fudan Univ, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Prev, Ctr Atmospher Chem Study, Shanghai, Peoples R China;
6.Ocean Univ China, Minist Educ China, Key Lab Marine Environm & Ecol, Qingdao, Shandong, Peoples R China
推荐引用方式
GB/T 7714
Sun, Jian,Fu, Joshua S.,Lynch, Jason A.,et al. Climate-driven exceedance of total (wet plus dry) nitrogen (N) plus sulfur (S) deposition to forest soil over the conterminous US[J]. 美国环保署,2017,5(6):560-576.
APA Sun, Jian,Fu, Joshua S.,Lynch, Jason A.,Huang, Kan,&Gao, Yang.(2017).Climate-driven exceedance of total (wet plus dry) nitrogen (N) plus sulfur (S) deposition to forest soil over the conterminous US.EARTHS FUTURE,5(6),560-576.
MLA Sun, Jian,et al."Climate-driven exceedance of total (wet plus dry) nitrogen (N) plus sulfur (S) deposition to forest soil over the conterminous US".EARTHS FUTURE 5.6(2017):560-576.
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