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DOI10.1016/j.apr.2017.02.003
Source identification of coarse particles in the Desert Southwest, USA using Positive Matrix Factorization
Clements, Andrea L.1,7; Fraser, Matthew P.2; Upadhyay, Nabin3,8; Herckes, Pierre3; Sundblom, Michael4; Lantz, Jeffrey5; Solomon, Paul A.6
发表日期2017-09-01
ISSN1309-1042
卷号8期号:5页码:873-884
英文摘要

The Desert Southwest Coarse Particulate Matter Study was undertaken to further our understanding of the spatial and temporal variability and sources of fine and coarse particulate matter (PM) in rural, arid, desert environments. Sampling was conducted between February 2009 and February 2010 in Pinal County, AZ near the town of Casa Grande where PM concentrations routinely exceed the U.S. National Ambient Air Quality Standards (NAAQS) for both PM10 and PM2.5. In this desert region, exceedances of the PM10 NAAQS are dominated by high coarse particle concentrations, a common occurrence in this region of the United States. This work expands on previously published measurements of PM mass and chemistry by examining the sources of fine and coarse particles and the relative contribution of each to ambient PM mass concentrations using the Positive Matrix Factorization receptor model (Clements et al., 2014).


Coarse particles within the region were apportioned to nine sources including primary biological aerosol particles (PBAPs - 25%), crustal material (20%), re-entrained road dust (11%), feedlot (11% at the site closest to a cattle feedlot), secondary particles (10%), boron-rich crustal material (9%), and transported soil (6%), with minor contributions from ammonium nitrate, and salt (considered to be NaCl). Fine particles within the region were apportioned to six sources including motor vehicles (37%), road dust (29%), lead-rich (10%), with minor contributions from brake wear, crustal material, and salt. These results can help guide local air pollution improvement strategies designed to reduce levels of PM to below the NAAQS. (C) 2017 Turkish National Committee for Air Pollution Research and Control. Production and hosting by Elsevier B.V. All rights reserved.


英文关键词Desert aerosols;Coarse particles;Positive matrix factorization;Crustal material;Feedlot;Road dust;Primary biological aerosol particles
语种英语
WOS记录号WOS:000417391200008
来源期刊ATMOSPHERIC POLLUTION RESEARCH
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/61084
作者单位1.Rice Univ, Dept Civil & Environm Engn, 6100 Main St,MS-519, Houston, TX 77005 USA;
2.Arizona State Univ, Sch Sustainable Engn & Built Environm, POB 873005, Tempe, AZ 85287 USA;
3.Arizona State Univ, Sch Mol Sci, POB 871604, Tempe, AZ 85287 USA;
4.Pinal Cty Air Qual Control Dist, 31 N Pinal St F, Florence, AZ 85132 USA;
5.US EPA, Off Air & Radiat, 4220 S Maryland Pkwy,Bld C, Las Vegas, NV 89119 USA;
6.US EPA, Off Res & Dev, 944 E Harmon Ave,Rm 235, Las Vegas, NV 89119 USA;
7.Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA;
8.ConocoPhillips Global Water Sustainabil Ctr, Qatar Sci & Technol Pk, Doha, Qatar
推荐引用方式
GB/T 7714
Clements, Andrea L.,Fraser, Matthew P.,Upadhyay, Nabin,et al. Source identification of coarse particles in the Desert Southwest, USA using Positive Matrix Factorization[J]. 美国环保署,2017,8(5):873-884.
APA Clements, Andrea L..,Fraser, Matthew P..,Upadhyay, Nabin.,Herckes, Pierre.,Sundblom, Michael.,...&Solomon, Paul A..(2017).Source identification of coarse particles in the Desert Southwest, USA using Positive Matrix Factorization.ATMOSPHERIC POLLUTION RESEARCH,8(5),873-884.
MLA Clements, Andrea L.,et al."Source identification of coarse particles in the Desert Southwest, USA using Positive Matrix Factorization".ATMOSPHERIC POLLUTION RESEARCH 8.5(2017):873-884.
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