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DOI10.5194/gmd-8-619-2015
Implementing marine organic aerosols into the GEOS-Chem model
Gantt, B.1; Johnson, M. S.2; Crippa, M.3; Prevot, A. S. H.3; Meskhidze, N.1
发表日期2015
ISSN1991-959X
卷号8期号:3页码:619-629
英文摘要

Marine-sourced organic aerosols (MOAs) have been shown to play an important role in tropospheric chemistry by impacting surface mass, cloud condensation nuclei, and ice nuclei concentrations over remote marine and coastal regions. In this work, an online marine primary organic aerosol emission parameterization, designed to be used for both global and regional models, was implemented into the GEOS-Chem (Global Earth Observing System Chemistry) model. The implemented emission scheme improved the large underprediction of organic aerosol concentrations in clean marine regions (normalized mean bias decreases from -79% when using the default settings to -12% when marine organic aerosols are added). Model predictions were also in good agreement (correlation coefficient of 0.62 and normalized mean bias of -36%) with hourly surface concentrations of MOAs observed during the summertime at an inland site near Paris, France. Our study shows that MOAs have weaker coastal-to-inland concentration gradients than sea-salt aerosols, leading to several inland European cities having > 10% of their surface submicron organic aerosol mass concentration with a marine source. The addition of MOA tracers to GEOS-Chem enabled us to identify the regions with large contributions of freshly emitted or aged aerosol having distinct physicochemical properties, potentially indicating optimal locations for future field studies.


语种英语
WOS记录号WOS:000352160200010
来源期刊GEOSCIENTIFIC MODEL DEVELOPMENT
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/60852
作者单位1.N Carolina State Univ, Dept Marine Earth & Atmospher Sci, Raleigh, NC 27695 USA;
2.NASA, Ames Res Ctr, Div Earth Sci, Moffett Field, CA 94035 USA;
3.Paul Scherrer Inst, Lab Atmospher Chem, Villigen, Switzerland
推荐引用方式
GB/T 7714
Gantt, B.,Johnson, M. S.,Crippa, M.,et al. Implementing marine organic aerosols into the GEOS-Chem model[J]. 美国环保署,2015,8(3):619-629.
APA Gantt, B.,Johnson, M. S.,Crippa, M.,Prevot, A. S. H.,&Meskhidze, N..(2015).Implementing marine organic aerosols into the GEOS-Chem model.GEOSCIENTIFIC MODEL DEVELOPMENT,8(3),619-629.
MLA Gantt, B.,et al."Implementing marine organic aerosols into the GEOS-Chem model".GEOSCIENTIFIC MODEL DEVELOPMENT 8.3(2015):619-629.
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