CCPortal
DOI10.1002/2017JD027057
Evaluation of the Community Multiscale Air Quality Model for Simulating Winter Ozone Formation in the Uinta Basin
Matichuk, Rebecca1; Tonnesen, Gail1; Luecken, Deborah2; Gilliam, Rob2; Napelenok, Sergey L.2; Baker, Kirk R.3; Schwede, Donna2; Murphy, Ben2; Helmig, Detlev4; Lyman, Seth N.5,6; Roselle, Shawn2
发表日期2017-12-27
ISSN2169-897X
卷号122期号:24页码:13545-13572
英文摘要

The Weather Research and Forecasting (WRF) and Community Multiscale Air Quality (CMAQ) models were used to simulate a 10day high-ozone episode observed during the 2013 Uinta Basin Winter Ozone Study (UBWOS). The baseline model had a large negative bias when compared to ozone (O-3) and volatile organic compound (VOC) measurements across the basin. Contrary to other wintertime Uinta Basin studies, predicted nitrogen oxides (NOx) were typically low compared to measurements. Increases to oil and gas VOC emissions resulted in O-3 predictions closer to observations, and nighttime O-3 improved when reducing the deposition velocity for all chemical species. Vertical structures of these pollutants were similar to observations on multiple days. However, the predicted surface layer VOC mixing ratios were generally found to be underestimated during the day and overestimated at night. While temperature profiles compared well to observations, WRF was found to have a warm temperature bias and too low nighttime mixing heights. Analyses of more realistic snow heat capacity in WRF to account for the warm bias and vertical mixing resulted in improved temperature profiles, although the improved temperature profiles seldom resulted in improved O-3 profiles. While additional work is needed to investigate meteorological impacts, results suggest that the uncertainty in the oil and gas emissions contributes more to the underestimation of O-3. Further, model adjustments based on a single site may not be suitable across all sites within the basin.


英文关键词photochemical grid models;CMAQ;WRF;winter ozone;air quality;oil and gas emissions
语种英语
WOS记录号WOS:000419950200026
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/60028
作者单位1.US EPA, Reg Off Partnerships & Regulatory Assistance 8, Air Program, Indoor Air Tox & Transportat Unit, Denver, CO 80202 USA;
2.US EPA, Off Res & Dev, Computat Exposure Div, Res Triangle Pk, NC USA;
3.US EPA, Off Air Qual Planning & Stand, Air Qual Assessment Div, Res Triangle Pk, NC USA;
4.Univ Colorado Boulder, Inst Artic & Alpine Res, Boulder, CO USA;
5.Utah State Univ, Bingham Res Ctr, Vernal, UT USA;
6.Utah State Univ, Dept Chem & Biochem, Vernal, UT USA
推荐引用方式
GB/T 7714
Matichuk, Rebecca,Tonnesen, Gail,Luecken, Deborah,et al. Evaluation of the Community Multiscale Air Quality Model for Simulating Winter Ozone Formation in the Uinta Basin[J]. 美国环保署,2017,122(24):13545-13572.
APA Matichuk, Rebecca.,Tonnesen, Gail.,Luecken, Deborah.,Gilliam, Rob.,Napelenok, Sergey L..,...&Roselle, Shawn.(2017).Evaluation of the Community Multiscale Air Quality Model for Simulating Winter Ozone Formation in the Uinta Basin.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,122(24),13545-13572.
MLA Matichuk, Rebecca,et al."Evaluation of the Community Multiscale Air Quality Model for Simulating Winter Ozone Formation in the Uinta Basin".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 122.24(2017):13545-13572.
条目包含的文件
条目无相关文件。
个性服务
推荐该条目
保存到收藏夹
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[Matichuk, Rebecca]的文章
[Tonnesen, Gail]的文章
[Luecken, Deborah]的文章
百度学术
百度学术中相似的文章
[Matichuk, Rebecca]的文章
[Tonnesen, Gail]的文章
[Luecken, Deborah]的文章
必应学术
必应学术中相似的文章
[Matichuk, Rebecca]的文章
[Tonnesen, Gail]的文章
[Luecken, Deborah]的文章
相关权益政策
暂无数据
收藏/分享

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。