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DOI10.5094/APR.2014.007
Chemical characterization of coarse particulate matter in the Desert Southwest - Pinal County Arizona, USA
Clements, Andrea L.1; Fraser, Matthew P.2; Upadhyay, Nabin3; Herckes, Pierre3; Sundblom, Michael4; Lantz, Jeffrey5; Solomon, Paul A.6
发表日期2014
ISSN1309-1042
卷号5期号:1页码:52-61
英文摘要

The Desert Southwest Coarse Particulate Matter Study was undertaken to further our understanding of ambient concentrations and the composition of fine and coarse particles in rural, arid environments. Sampling was conducted in Pinal County, Arizona between February 2009 and February 2010. The goals of this study were to: (1) chemically characterize the coarse and fine fraction of the ambient particulate matter in terms of mass, ions, elements, bulk organic and elemental carbon; (2) examine the temporal and spatial variability of particles within the area using a series of three sampling locations and use this information to determine the contribution of local vs. regional sources; (3) collect, re-suspend, and chemically characterize various crustal sources within the area to identify differences which may isolate them (crustal sources) as independent sources, and; (4) use a receptor based modeling approach to identify particle sources and the relative impact of each on ambient PM concentrations. This work reviews the study objectives, design, site descriptions, and measurement techniques relevant to this research effort and presents the general characteristics of PM during the study period. This unique dataset will support efforts to reduce PM10 and PM2.5 concentrations in the area to below the National Ambient Air Quality Standards (NAAQS) for these pollutants.


Coarse particle concentrations are, on average, approximately 5 times fine particle mass concentrations within the region. Coarse particle concentrations in Pinal County are highest during spring and fall seasons, consistent with the tilling and harvesting seasons while fine particles concentrations are highest during fall. Crustal material is the dominant component of coarse particle composition, representing 50% of the mass on average followed closely by organic matter representing 15%. Fine particles still contain a significant crustal fraction (30%) but organic matter dominates at 37% of the particle mass.


英文关键词Desert aerosols;coarse particles;fine particles;chemical composition
语种英语
WOS记录号WOS:000331398400007
来源期刊ATMOSPHERIC POLLUTION RESEARCH
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59699
作者单位1.Rice Univ, Dept Civil & Environm Engn, Houston, TX 77005 USA;
2.Arizona State Univ, Sch Sustainabil & Built Environm, Tempe, AZ 85287 USA;
3.Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA;
4.Pinal Cty Air Qual Control Dist, Florence, AZ 85132 USA;
5.US EPA, Off Air & Radiat, Las Vegas, NV 89193 USA;
6.US EPA, Off Res & Dev, Las Vegas, NV 89119 USA
推荐引用方式
GB/T 7714
Clements, Andrea L.,Fraser, Matthew P.,Upadhyay, Nabin,et al. Chemical characterization of coarse particulate matter in the Desert Southwest - Pinal County Arizona, USA[J]. 美国环保署,2014,5(1):52-61.
APA Clements, Andrea L..,Fraser, Matthew P..,Upadhyay, Nabin.,Herckes, Pierre.,Sundblom, Michael.,...&Solomon, Paul A..(2014).Chemical characterization of coarse particulate matter in the Desert Southwest - Pinal County Arizona, USA.ATMOSPHERIC POLLUTION RESEARCH,5(1),52-61.
MLA Clements, Andrea L.,et al."Chemical characterization of coarse particulate matter in the Desert Southwest - Pinal County Arizona, USA".ATMOSPHERIC POLLUTION RESEARCH 5.1(2014):52-61.
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