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DOI10.4209/aaqr.2013.07.0253
Size-Differentiated Chemical Composition of Re-Suspended Soil Dust from the Desert Southwest United States
Upadhyay, Nabin1; Clements, Andrea L.2,3; Fraser, Matthew P.2,3; Sundblom, Michael4; Solomon, Paul5; Herckes, Pierre1
发表日期2015-04-01
ISSN1680-8584
卷号15期号:2页码:387-U40
英文摘要

As part of the Desert Southwest Coarse Particulate Matter Study which characterized the composition of fine and coarse particulate matter in Pinal County, AZ during 2010-2011, several source samples were collected from several different soil types to assist in source apportionment analysis of the study results. Soil types included native desert soils, agricultural soils (crop farming), dirt-road material adjacent to agricultural areas, paved road dusts, dirt road material from within and adjacent to a cattle feedlot, and material from an active cattle feedlot. Following laboratory resuspension of the soil, size-segregated PM2.5 and PM10 fractions for each source type were collected on filters and characterized for mass, ions, OC, EC, and trace elements. While there are unique chemical compositions of soils in the region (e.g., high As and Sb) that reiterate the importance of using local source profiles (e.g., native soils) as compared to Upper Continental Crust or soil profiles from other regions in receptor modeling studies. The study also provides new insights into the impact of land-use modification on source emission profiles. Specifically, high OC and PO43- are found in material representative of local cattle feedlot activities while elevated Cu, Sb and Zn are found from sources impacted by motor vehicle traffic. Results of the study indicate that the local native soil composition is only slightly modified by agricultural activities and this study provides the chemical composition of both native and agricultural soil for source apportionment studies in the Desert Southwest.


英文关键词Cattle feedlots;Dirt road dust;Paved road dust;Agricultural soils;Source characterization
语种英语
WOS记录号WOS:000353175300003
来源期刊AEROSOL AND AIR QUALITY RESEARCH
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59510
作者单位1.Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA;
2.Rice Univ, Dept Civil & Environm Engn, Houston, TX 77005 USA;
3.Arizona State Univ, Sch Sustainable Engn & Built Environm, Tempe, AZ 85287 USA;
4.Pinal Cty Air Qual Control Dist, Florence, AZ 85232 USA;
5.US EPA, Off Res & Dev, Las Vegas, NV 89119 USA
推荐引用方式
GB/T 7714
Upadhyay, Nabin,Clements, Andrea L.,Fraser, Matthew P.,et al. Size-Differentiated Chemical Composition of Re-Suspended Soil Dust from the Desert Southwest United States[J]. 美国环保署,2015,15(2):387-U40.
APA Upadhyay, Nabin,Clements, Andrea L.,Fraser, Matthew P.,Sundblom, Michael,Solomon, Paul,&Herckes, Pierre.(2015).Size-Differentiated Chemical Composition of Re-Suspended Soil Dust from the Desert Southwest United States.AEROSOL AND AIR QUALITY RESEARCH,15(2),387-U40.
MLA Upadhyay, Nabin,et al."Size-Differentiated Chemical Composition of Re-Suspended Soil Dust from the Desert Southwest United States".AEROSOL AND AIR QUALITY RESEARCH 15.2(2015):387-U40.
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