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DOI10.1016/j.apr.2015.08.003
Estimating ozone and secondary PM2.5 impacts from hypothetical single source emissions in the central and eastern United States
Baker, Kirk R.1; Kotchenruther, Robert A.2; Hudman, Rynda C.3
发表日期2016
ISSN1309-1042
卷号7期号:1页码:122-133
英文摘要

Secondary pollutant impacts from emissions of single sources may need to be assessed to satisfy a variety of regulatory requirements including the Clean Air Act New Source Review and Prevention of Significant Deterioration programs and the National Environmental Policy Act. In this work, single source impacts on O-3 and secondary PM2.5 are estimated with annual 2011 photochemical grid model simulations where new hypothetical sources are added to the central and eastern United States with varying precursor emission rates and emission release heights. Impacts from these hypothetical sources are tracked with photochemical grid model source apportionment. Single source impacts on downwind 8-hr maximum O-3 tend to increase as emissions of NOX or VOC increase. Downwind impacts on PM2.5 sulfate and nitrate also tend to increase as emissions of SO2 and NOX increase. For all secondary pollutants, impacts from these hypothetical sources tend to decrease as distance from the source increases. However, peak impacts on O-3 and secondary PM2.5 are not at the facility fence-line but typically within 50-100 km depending on the emissions rate, precursor pollutant, and emissions release point. Downwind impacts are not uniform directionally from these sources due to varying downwind availability of chemical reactants and prevailing meteorology. Peak impacts for O-3 (similar to 15 ppb) and PM2.5 sulfate (similar to 8 mu g/m(3)) were within 50 km of these hypothetical sources and peak impacts for PM2.5 nitrate (similar to 1 mu g/m(3)) were within 125 km. The daily maximum 8-hr O-3 and maximum daily average PM2.5 sulfate and nitrate ion impacts for the new hypothetical sources modeled here are generally consistent with those reported in literature. Additional assessments of single source impacts on secondary pollutants are still needed to provide a more comprehensive assessment of different source types and source environments. Copyright (C) 2015 Turkish National Committee for Air Pollution Research and Control. Production and hosting by Elsevier B.V. All rights reserved.


英文关键词Photochemical model;Ozone;PM;Single source;Source apportionment
语种英语
WOS记录号WOS:000372528400015
来源期刊ATMOSPHERIC POLLUTION RESEARCH
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59459
作者单位1.US EPA, Res Triangle Pk, NC 27711 USA;
2.US EPA, Seattle, WA USA;
3.US EPA, San Francisco, CA USA
推荐引用方式
GB/T 7714
Baker, Kirk R.,Kotchenruther, Robert A.,Hudman, Rynda C.. Estimating ozone and secondary PM2.5 impacts from hypothetical single source emissions in the central and eastern United States[J]. 美国环保署,2016,7(1):122-133.
APA Baker, Kirk R.,Kotchenruther, Robert A.,&Hudman, Rynda C..(2016).Estimating ozone and secondary PM2.5 impacts from hypothetical single source emissions in the central and eastern United States.ATMOSPHERIC POLLUTION RESEARCH,7(1),122-133.
MLA Baker, Kirk R.,et al."Estimating ozone and secondary PM2.5 impacts from hypothetical single source emissions in the central and eastern United States".ATMOSPHERIC POLLUTION RESEARCH 7.1(2016):122-133.
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