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DOI10.1016/j.watres.2017.07.037
Linking terrestrial phosphorus inputs to riverine export across the United States
Metson, Genevieve S.1,2,3; Lin, Jiajia1,3; Harrison, John A.2; Compton, Jana E.3
发表日期2017-11-01
ISSN0043-1354
卷号124页码:177-191
英文摘要

Humans have greatly accelerated phosphorus (P) flows from land to aquatic ecosystems, causing eutrophication, harmful algal blooms, and hypoxia. A variety of statistical and mechanistic models have been used to explore the relationship between P management on land and P losses to waterways, but our ability to predict P losses from watersheds often relies on small scale catchment studies, where detailed measurements can be made, or global scale models that that are often too coarse-scaled to be used directly in the management decision-making process. Here we constructed spatially explicit datasets of terrestrial P inputs and outputs across the conterminous U.S. (CONUS) for 2012. We use this dataset to improve understanding of P sources and balances at the national scale and to investigate whether well standardized input data at the continental scale can be used to improve predictions of hydrologic P export from watersheds across the U.S. We estimate that in 2012 agricultural lands received 0.19 Tg more P as fertilizer and confined manure than was harvested in major crops. Approximately 0.06 Tg P was lost to waterways as sewage and detergent nationally based on per capita loads in 2012. We compared two approaches for calculating non-agricultural P waste export to waterways, and found that estimates based on per capita P loads from sewage and detergent were 50% greater than Discharge Monitoring Report Pollutant Loading Tool. This suggests that the tool is likely underestimating P export in waste the CONUS scale. TP and DIP concentrations and TP yields were generally correlated more strongly with runoff than with P inputs or P balances, but even the relationships between runoff and P export were weak. Including P inputs as independent variables increased the predictive capacity of the best-fit models by at least 20%, but together inputs and runoff explained 40% of the variance in P concentration and 46-54% of the variance in P yield. By developing and applying a high-resolution P budget for the CONUS this study confirms that both hydrology and P inputs and sinks play important roles in aquatic P loading across a wide range of environments. (C) 2017 Elsevier Ltd. All rights reserved.


英文关键词Phosphorus;Water quality;Agriculture;Sewage
语种英语
WOS记录号WOS:000412251500017
来源期刊WATER RESEARCH
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59148
作者单位1.Natl Acad Sci, Natl Res Council, Washington, DC 20001 USA;
2.Washington State Univ, Sch Environm, Vancouver, WA 98686 USA;
3.US Environm Protect Agcy, Western Ecol Div, Off Res & Dev, 200 SW 35th St, Corvallis, OR 97333 USA
推荐引用方式
GB/T 7714
Metson, Genevieve S.,Lin, Jiajia,Harrison, John A.,et al. Linking terrestrial phosphorus inputs to riverine export across the United States[J]. 美国环保署,2017,124:177-191.
APA Metson, Genevieve S.,Lin, Jiajia,Harrison, John A.,&Compton, Jana E..(2017).Linking terrestrial phosphorus inputs to riverine export across the United States.WATER RESEARCH,124,177-191.
MLA Metson, Genevieve S.,et al."Linking terrestrial phosphorus inputs to riverine export across the United States".WATER RESEARCH 124(2017):177-191.
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