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DOI10.2166/wst.2017.033
A greenhouse gas source of surprising significance: anthropogenic CO2 emissions from use of methanol in sewage treatment
Willis, John L.1,2; Al-Omari, Ahmed3; Bastian, Robert4; Brower, Bill3; DeBarbadillo, Christine3; Murthy, Sudhir3; Peot, Christopher3; Yuan, Zhiguo1
发表日期2017-05-01
ISSN0273-1223
卷号75期号:9页码:1997-2012
英文摘要

The impact of methanol (CH3OH) as a source of anthropogenic carbon dioxide (CO2) in denitrification at wastewater treatment plants (WWTPs) has never been quantified. CH3OH is the most commonly purchased carbon source for sewage denitrification. Until recently, greenhouse gas (GHG) reporting protocols consistently ignored the liberation of anthropogenic CO2 attributable to CH3OH. This oversight can likely be attributed to a simplifying notion that CO2 produced through activated-sludge-process respiration is biogenic because most raw-sewage carbon is un-sequestered prior to entering a WWTP. Instead, a biogenic categorization cannot apply to fossil-fuel-derived carbon sources like CH3OH. This paper provides a summary of how CH3OH use at DC Water's Blue Plains Advanced Wastewater Treatment Plant (AWTP; Washington, DC, USA) amounts to 60 to 85% of the AWTP's Scope-1 emissions. The United States Environmental Protection Agency and Water Environment Federation databases suggest that CH3OH CO2 likely represents one quarter of all Scope-1 GHG emissions attributable to sewage treatment in the USA. Finally, many alternatives to CH3OH use exist and are discussed.


英文关键词anthropogenic greenhouse gas;global-warming mitigation;methanol;methodology;nitrogen removal;sewage treatment
语种英语
WOS记录号WOS:000401150500002
来源期刊WATER SCIENCE AND TECHNOLOGY
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/59070
作者单位1.Univ Queensland, Adv Water Management Ctr, Gehrmann Bldg Level 4, St Lucia, Qld 4072, Australia;
2.Brown & Caldwell, 990 Hammond Dr,Suite 400, Atlanta, GA 30326 USA;
3.DC Water, 5000 Overlook Ave SW, Washington, DC 20032 USA;
4.US EPA, Off Wastewater Management, 1200 Penn Ave NW, Washington, DC 20460 USA
推荐引用方式
GB/T 7714
Willis, John L.,Al-Omari, Ahmed,Bastian, Robert,et al. A greenhouse gas source of surprising significance: anthropogenic CO2 emissions from use of methanol in sewage treatment[J]. 美国环保署,2017,75(9):1997-2012.
APA Willis, John L..,Al-Omari, Ahmed.,Bastian, Robert.,Brower, Bill.,DeBarbadillo, Christine.,...&Yuan, Zhiguo.(2017).A greenhouse gas source of surprising significance: anthropogenic CO2 emissions from use of methanol in sewage treatment.WATER SCIENCE AND TECHNOLOGY,75(9),1997-2012.
MLA Willis, John L.,et al."A greenhouse gas source of surprising significance: anthropogenic CO2 emissions from use of methanol in sewage treatment".WATER SCIENCE AND TECHNOLOGY 75.9(2017):1997-2012.
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