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DOI10.1016/j.atmosenv.2015.12.048
Investigating the impact of local urban sources on total atmospheric mercury wet deposition in Cleveland, Ohio, USA
Lynam, Mary M.1; Dvonch, J. Timothy1; Barres, James A.1; Landis, Matthew S.2; Kamal, Ali S.2,3
发表日期2016-02-01
ISSN1352-2310
卷号127页码:262-271
英文摘要

Event-based precipitation samples were collected at a downtown industrial and a predominantly upwind rural location in the Cleveland, Ohio metropolitan area from July 2009 through December 2010 to investigate the potential local total mercury (Hg) wet deposition enhancement in a region with a high concentration of coal combustion sources. Total Hg wet deposition for the 18 -month period was 6.8 mu g m(-2) (n = 81) at the rural site and 10.7 mu g m(-2) (n = 98) at the urban site demonstrating a significant (p = 0.046) 37% enhancement in deposition between the two sites. Large deposition events (>0.2 mu g m(-2)) occurred predominantly from May through October (n = 16 (urban), n = 10 (rural)) and represented from 2 to 8% of total 18-month deposition per event. At the downtown urban site, the average Hg precipitation concentration was 53% higher for these large deposition events. Concurrently measured precipitation events delivered in aggregate 2.4 times more total Hg wet deposition to the urban site compared to the rural site. Hg rainfall concentrations for concurrent events with similar precipitation depth were 2-4 times higher at the urban site and suggest scavenging of local Hg emissions. Further evaluation of these events revealed 83% more total Hg deposition at the urban site from January to December 2010 compared to July to December 2009, while there was 26% more at the rural site during these same time periods. The larger increase in deposition at the urban site in 2010 may be evidence of increased local emissions from sources that were known to be offline during this study period because of an economic recession. (C) 2015 Elsevier Ltd. All rights reserved.


英文关键词Mercury deposition network;Meteorological case study;Lake Erie
语种英语
WOS记录号WOS:000370770700030
来源期刊ATMOSPHERIC ENVIRONMENT
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/58603
作者单位1.Univ Michigan, Air Qual Lab, Ann Arbor, MI 48109 USA;
2.US EPA, Off Res & Dev, Res Triangle Pk, NC 27711 USA;
3.US EPA, Off Air Qual Planning & Stand, Res Triangle Pk, NC 27711 USA
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Lynam, Mary M.,Dvonch, J. Timothy,Barres, James A.,et al. Investigating the impact of local urban sources on total atmospheric mercury wet deposition in Cleveland, Ohio, USA[J]. 美国环保署,2016,127:262-271.
APA Lynam, Mary M.,Dvonch, J. Timothy,Barres, James A.,Landis, Matthew S.,&Kamal, Ali S..(2016).Investigating the impact of local urban sources on total atmospheric mercury wet deposition in Cleveland, Ohio, USA.ATMOSPHERIC ENVIRONMENT,127,262-271.
MLA Lynam, Mary M.,et al."Investigating the impact of local urban sources on total atmospheric mercury wet deposition in Cleveland, Ohio, USA".ATMOSPHERIC ENVIRONMENT 127(2016):262-271.
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