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DOI | 10.1038/s41598-017-06981-8 |
Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions | |
Xie, Mingjie1,2; Hays, Michael D.2; Holder, Amara L.2 | |
发表日期 | 2017-08-04 |
ISSN | 2045-2322 |
卷号 | 7 |
英文摘要 | Light-absorbing organic carbon (OC), also termed brown carbon (BrC), from laboratory-based biomass burning (BB) has been studied intensively to understand the contribution of BB to radiative forcing. However, relatively few measurements have been conducted on field-based BB and even fewer measurements have examined BrC from anthropogenic combustion sources like motor vehicle emissions. In this work, the light absorption of methanol-extractable OC from prescribed and laboratory BB and gasoline vehicle emissions was examined using spectrophotometry. The light absorption of methanol extracts showed a strong wavelength dependence for both BB and gasoline vehicle emissions. The mass absorption coefficients at 365 nm (MAC(365), m(2) g(-1)C) - used as a measurement proxy for BrC - were significantly correlated (p < 0.05) to the elemental carbon (EC)/OC ratios when examined by each BB fuel type. No significant correlation was observed when pooling fuels, indicating that both burn conditions and fuel types may impact BB BrC characteristics. The average MAC(365) of gasoline vehicle emission samples is 0.62 +/- 0.76 m(2) g(-1)C, which is similar in magnitude to the BB samples (1.27 +/- 0.76 m(2) g(-1)C). These results suggest that in addition to BB, gasoline vehicle emissions may also be an important BrC source in urban areas. |
语种 | 英语 |
WOS记录号 | WOS:000406980800057 |
来源期刊 | SCIENTIFIC REPORTS |
来源机构 | 美国环保署 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/58427 |
作者单位 | 1.ORISE, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA; 2.US EPA, Off Res & Dev, Natl Risk Management Res Lab, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA |
推荐引用方式 GB/T 7714 | Xie, Mingjie,Hays, Michael D.,Holder, Amara L.. Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions[J]. 美国环保署,2017,7. |
APA | Xie, Mingjie,Hays, Michael D.,&Holder, Amara L..(2017).Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions.SCIENTIFIC REPORTS,7. |
MLA | Xie, Mingjie,et al."Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions".SCIENTIFIC REPORTS 7(2017). |
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