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DOI10.1038/s41598-017-06981-8
Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions
Xie, Mingjie1,2; Hays, Michael D.2; Holder, Amara L.2
发表日期2017-08-04
ISSN2045-2322
卷号7
英文摘要

Light-absorbing organic carbon (OC), also termed brown carbon (BrC), from laboratory-based biomass burning (BB) has been studied intensively to understand the contribution of BB to radiative forcing. However, relatively few measurements have been conducted on field-based BB and even fewer measurements have examined BrC from anthropogenic combustion sources like motor vehicle emissions. In this work, the light absorption of methanol-extractable OC from prescribed and laboratory BB and gasoline vehicle emissions was examined using spectrophotometry. The light absorption of methanol extracts showed a strong wavelength dependence for both BB and gasoline vehicle emissions. The mass absorption coefficients at 365 nm (MAC(365), m(2) g(-1)C) - used as a measurement proxy for BrC - were significantly correlated (p < 0.05) to the elemental carbon (EC)/OC ratios when examined by each BB fuel type. No significant correlation was observed when pooling fuels, indicating that both burn conditions and fuel types may impact BB BrC characteristics. The average MAC(365) of gasoline vehicle emission samples is 0.62 +/- 0.76 m(2) g(-1)C, which is similar in magnitude to the BB samples (1.27 +/- 0.76 m(2) g(-1)C). These results suggest that in addition to BB, gasoline vehicle emissions may also be an important BrC source in urban areas.


语种英语
WOS记录号WOS:000406980800057
来源期刊SCIENTIFIC REPORTS
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/58427
作者单位1.ORISE, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA;
2.US EPA, Off Res & Dev, Natl Risk Management Res Lab, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA
推荐引用方式
GB/T 7714
Xie, Mingjie,Hays, Michael D.,Holder, Amara L.. Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions[J]. 美国环保署,2017,7.
APA Xie, Mingjie,Hays, Michael D.,&Holder, Amara L..(2017).Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions.SCIENTIFIC REPORTS,7.
MLA Xie, Mingjie,et al."Light-absorbing organic carbon from prescribed and laboratory biomass burning and gasoline vehicle emissions".SCIENTIFIC REPORTS 7(2017).
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