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DOI10.1002/2015JD024321
Particulate matter and black carbon optical properties and emission factors from prescribed fires in the southeastern United States
Holder, Amara L.1; Hagler, Gayle S. W.1; Aurell, Johanna2; Hays, Michael D.1; Gullett, Brian K.1
发表日期2016-04-16
ISSN2169-897X
卷号121期号:7页码:3465-3483
英文摘要

Aerosol optical properties of biomass burning emissions are critical parameters determining how these emissions impact the Earth's climate. Despite their importance, field measurements of aerosol optical properties from fires remain scarce. Aerosol emissions from prescribed fires of forested and grass plots in the southeastern United States were measured and compared to emissions from laboratory simulations. Fine particulate matter (PM2.5), black carbon (BC), and aerosol light scattering and absorption were characterized for all fires. Refractory BC emission factors (EFs) measured at ground level (similar to 2m) were 0.760.15g/kg, comparable to the 0.930.32g/kg measured aloft (similar to 100-600m). However, PM EFs measured by aircraft were only 18% (5.42.0g/kg) of those measured on the ground (28.89.8g/kg). Such large differences in PM EFs for the same fire have not been previously reported and may plausibly be due to the differing particle measurement methodologies being applied but also likely related to partitioning of organic compounds to the gas phase as the plume dilutes aloft. Higher PM EFs on the ground may also be related to a higher contribution from smoldering combustion. The absorption angstrom ngstrom exponents ((a)) for the high intensity South Carolina fires were 3.92 +/- 0.6, which was larger than prescribed forest fire in Florida (2.84) and the grass fire in Florida (2.71), implying a larger absorption contribution from brown carbon from higher-intensity fires. Aerosol optical properties from laboratory simulations did not represent field measurements.


英文关键词biomass burning;black carbon mixing state;aerosol optical properties;size distributions;brown carbon
语种英语
WOS记录号WOS:000375120200024
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
来源机构美国环保署
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/57726
作者单位1.US EPA, Off Res & Dev, Res Triangle Pk, NC 27711 USA;
2.Univ Dayton, Res Inst, Energy Technol & Mat Div, Dayton, OH 45469 USA
推荐引用方式
GB/T 7714
Holder, Amara L.,Hagler, Gayle S. W.,Aurell, Johanna,et al. Particulate matter and black carbon optical properties and emission factors from prescribed fires in the southeastern United States[J]. 美国环保署,2016,121(7):3465-3483.
APA Holder, Amara L.,Hagler, Gayle S. W.,Aurell, Johanna,Hays, Michael D.,&Gullett, Brian K..(2016).Particulate matter and black carbon optical properties and emission factors from prescribed fires in the southeastern United States.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,121(7),3465-3483.
MLA Holder, Amara L.,et al."Particulate matter and black carbon optical properties and emission factors from prescribed fires in the southeastern United States".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 121.7(2016):3465-3483.
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