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DOI10.1016/j.scitotenv.2023.169639
A comparison of Tier 1, 2, and 3 methods for quantifying nitrous oxide emissions from soils amended with biosolids
发表日期2024
ISSN0048-9697
EISSN1879-1026
起始页码915
卷号915
英文摘要Municipal biosolids are a nitrogen (N)-rich agricultural fertilizer which may emit nitrous oxide (N2O) after rainfall events. Due to sparse empirical data, there is a lack of biosolids-specific N2O emission factors to determine how land-applied biosolids contribute to the national greenhouse gas inventory. This study estimated N2O emissions from biosolids-amended land in Canada using Tier 1, Tier 2 (Canadian), and Tier 3 (Denitrification and Decomposition model [DNDC]) methodologies recommended by the Intergovernmental Panel on Climate Change (IPCC). Field data was from replicated plots at 8 site-years between 2017 and 2019 in the provinces of Quebec, Nova Scotia and Alberta, Canada, representing three distinct ecozones. Municipal biosolids were the major N source for the crop, applied as mesophilic anaerobically digested biosolids, composted biosolids, or alkaline-stabilized biosolids alone or combined with an equal amount of urea-N fertilizer to meet the crop N requirements. Fluxes of N2O were measured during the growing season with manual chambers and compared to N2O emissions estimated using the IPCC methods. In all site-years, the mean emission of N2O in the growing season was greater with digested biosolids than other biosolids sources or urea fertilizer alone. The emissions of N2O in the growing season were similar with composted or alkaline-stabilized biosolids, and no greater than the unfertilized control. The best estimates of N2O emissions, relative to measured values, were with the Tier 3 > adapted Tier 2 with biosolids-specific correction factors > standard Tier 2 = Tier 1 methods of the IPCC, according to the root mean square error statistic. The Tier 3 IPCC method was the best estimator of N2O emissions in the Canadian ecozones evaluated in this study. These results will be used to improve methods for estimating N2O emissions from agricultural soils amended with biosolids and to generate more accurate GHG inventories.
英文关键词DNDC; N2O emissions; IPCC Tier 3; Nitrogen fertilizer; National GHG inventory
语种英语
WOS研究方向Environmental Sciences & Ecology
WOS类目Environmental Sciences
WOS记录号WOS:001168938300001
来源期刊SCIENCE OF THE TOTAL ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/304398
作者单位McGill University; Agriculture & Agri Food Canada; Environment & Climate Change Canada; Dalhousie University; University of Alberta; McGill University
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GB/T 7714
. A comparison of Tier 1, 2, and 3 methods for quantifying nitrous oxide emissions from soils amended with biosolids[J],2024,915.
APA (2024).A comparison of Tier 1, 2, and 3 methods for quantifying nitrous oxide emissions from soils amended with biosolids.SCIENCE OF THE TOTAL ENVIRONMENT,915.
MLA "A comparison of Tier 1, 2, and 3 methods for quantifying nitrous oxide emissions from soils amended with biosolids".SCIENCE OF THE TOTAL ENVIRONMENT 915(2024).
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