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DOI10.5194/acp-24-4949-2024
Summertime tropospheric ozone source apportionment study in the Madrid region (Spain)
de la Paz, David; Borge, Rafael; de Andres, Juan Manuel; Tovar, Luis; Sarwar, Golam; Napelenok, Sergey L.
发表日期2024
ISSN1680-7316
EISSN1680-7324
起始页码24
结束页码8
卷号24期号:8
英文摘要The design of emission abatement measures to effectively reduce high ground-level ozone ( O 3 ) concentrations in urban areas is very complex. In addition to the strongly non-linear chemistry of this secondary pollutant, precursors can be released by a variety of sources in different regions, and locally produced O 3 is mixed with that transported from the regional or continental scales. All of these processes depend also on the specific meteorological conditions and topography of the study area. Consequently, high-resolution comprehensive modeling tools are needed to understand the drivers of photochemical pollution and to assess the potential of local strategies to reduce adverse impacts from high tropospheric O 3 levels. In this study, we apply the Integrated Source Apportionment Method (ISAM) implemented in the Community Multiscale Air Quality (CMAQ v5.3.2) model to investigate the origin of summertime O 3 in the Madrid region (Spain). Consistent with previous studies, our results confirm that O 3 levels are dominated by non-local contributions, representing around 70 % of mean values across the region. Nonetheless, precursors emitted by local sources, mainly road traffic, play a more important role during O 3 peaks, with contributions as high as 25 ppb. The potential impact of local measures is higher under unfavorable meteorological conditions associated with regional accumulation patterns. These findings suggest that this modeling system may be used in the future to simulate the potential outcomes of specific emission abatement measures to prevent high- O 3 episodes in the Madrid metropolitan area.
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS记录号WOS:001209207000001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/298000
作者单位Universidad Politecnica de Madrid; United States Environmental Protection Agency
推荐引用方式
GB/T 7714
de la Paz, David,Borge, Rafael,de Andres, Juan Manuel,et al. Summertime tropospheric ozone source apportionment study in the Madrid region (Spain)[J],2024,24(8).
APA de la Paz, David,Borge, Rafael,de Andres, Juan Manuel,Tovar, Luis,Sarwar, Golam,&Napelenok, Sergey L..(2024).Summertime tropospheric ozone source apportionment study in the Madrid region (Spain).ATMOSPHERIC CHEMISTRY AND PHYSICS,24(8).
MLA de la Paz, David,et al."Summertime tropospheric ozone source apportionment study in the Madrid region (Spain)".ATMOSPHERIC CHEMISTRY AND PHYSICS 24.8(2024).
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