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DOI | 10.1021/acs.est.3c10307 |
Underestimation of Thermogenic Methane Emissions in New York City | |
Pitt, Joseph R.; Lopez-Coto, Israel; Karion, Anna; Hajny, Kristian D.; Tomlin, Jay; Kaeser, Robert; Jayarathne, Thilina; Stirm, Brian H.; Floerchinger, Cody R.; Loughner, Christopher P.; Commane, Roisin; Gately, Conor K.; Hutyra, Lucy R.; Gurney, Kevin R.; Roest, Geoffrey S.; Liang, Jianming; Gourdji, Sharon; Mueller, Kimberly L.; Whetstone, James R.; Shepson, Paul B. | |
发表日期 | 2024 |
ISSN | 0013-936X |
EISSN | 1520-5851 |
起始页码 | 58 |
结束页码 | 21 |
卷号 | 58期号:21 |
英文摘要 | Recent studies have shown that methane emissions are underestimated by inventories in many US urban areas. This has important implications for climate change mitigation policy at the city, state, and national levels. Uncertainty in both the spatial distribution and sectoral allocation of urban emissions can limit the ability of policy makers to develop appropriately focused emission reduction strategies. Top-down emission estimates based on atmospheric greenhouse gas measurements can help to improve inventories and inform policy decisions. This study presents a new high-resolution (0.02 x 0.02 degrees) methane emission inventory for New York City and its surrounding area, constructed using the latest activity data, emission factors, and spatial proxies. The new high-resolution inventory estimates of methane emissions for the New York-Newark urban area are 1.3 times larger than those for the gridded Environmental Protection Agency inventory. We used aircraft mole fraction measurements from nine research flights to optimize the high-resolution inventory emissions within a Bayesian inversion. These sectorally optimized emissions show that the high-resolution inventory still significantly underestimates methane emissions within the New York-Newark urban area, primarily because it underestimates emissions from thermogenic sources (by a factor of 2.3). This suggests that there remains a gap in our process-based understanding of urban methane emissions. |
英文关键词 | urban emissions; greenhouse gas emissions; methane; airborne greenhouse gas measurements; Bayesian inverse modeling; emissions inventory development; New York City |
语种 | 英语 |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
WOS类目 | Engineering, Environmental ; Environmental Sciences |
WOS记录号 | WOS:001225259200001 |
来源期刊 | ENVIRONMENTAL SCIENCE & TECHNOLOGY |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/296707 |
作者单位 | State University of New York (SUNY) System; State University of New York (SUNY) Stony Brook; University of Bristol; National Institute of Standards & Technology (NIST) - USA; Purdue University System; Purdue University; Bristol-Myers Squibb; Purdue University System; Purdue University; Harvard University; National Oceanic Atmospheric Admin (NOAA) - USA; Columbia University; Boston University; Northern Arizona University |
推荐引用方式 GB/T 7714 | Pitt, Joseph R.,Lopez-Coto, Israel,Karion, Anna,et al. Underestimation of Thermogenic Methane Emissions in New York City[J],2024,58(21). |
APA | Pitt, Joseph R..,Lopez-Coto, Israel.,Karion, Anna.,Hajny, Kristian D..,Tomlin, Jay.,...&Shepson, Paul B..(2024).Underestimation of Thermogenic Methane Emissions in New York City.ENVIRONMENTAL SCIENCE & TECHNOLOGY,58(21). |
MLA | Pitt, Joseph R.,et al."Underestimation of Thermogenic Methane Emissions in New York City".ENVIRONMENTAL SCIENCE & TECHNOLOGY 58.21(2024). |
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