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DOI | 10.1016/j.jhazmat.2024.134043 |
Natural organic small molecules promote the aging of plastic wastes and refractory carbon decomposition in water | |
发表日期 | 2024 |
ISSN | 0304-3894 |
EISSN | 1873-3336 |
起始页码 | 469 |
卷号 | 469 |
英文摘要 | Microplastics and nanoplastics are ubiquitous in rivers and undergo environmental aging. However, the molecular mechanisms of plastic aging and the in-depth effects of aging on ecological functions remain unclear in waters. The synergies of microplastics and nanoplastics (polystyrene as an example) with natural organic small molecules (e.g., natural hyaluronic acid and vitamin C related to biological tissue decomposition) are the key to producing radicals (center dot OH and center dot C). The radicals promote the formation of bubbles on plastic surfaces and generate derivatives of plastics such as monomer and dimer styrene. Nanoplastics are easier to age than microplastics. Pristine plastics inhibit the microbial Shannon diversity index and evenness, but the opposite results are observed for aging plastics. Pristine plastics curb pectin decomposition (an indicator of plant-originated refractory carbon), but aging plastics promote pectin decomposition. Microplastics and nanoplastics undergoing aging processes enhance the carbon biogeochemical cycle. For example, the increased carbohydrate active enzyme diversity, especially the related glycoside hydrolase and functional species Pseudomonas and Clostridium, contributes to refractory carbon decomposition. Different from the well-studied toxicity and aging of plastic pollutants, this study connects plastic pollutants with biological tissue decomposition, biodiversity and climate change together in rivers. |
英文关键词 | Microplastics; Nanoplastics; Carbon cycle; Microbial function; Carbon decomposition |
语种 | 英语 |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
WOS类目 | Engineering, Environmental ; Environmental Sciences |
WOS记录号 | WOS:001219140700001 |
来源期刊 | JOURNAL OF HAZARDOUS MATERIALS |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/294584 |
作者单位 | Nankai University |
推荐引用方式 GB/T 7714 | . Natural organic small molecules promote the aging of plastic wastes and refractory carbon decomposition in water[J],2024,469. |
APA | (2024).Natural organic small molecules promote the aging of plastic wastes and refractory carbon decomposition in water.JOURNAL OF HAZARDOUS MATERIALS,469. |
MLA | "Natural organic small molecules promote the aging of plastic wastes and refractory carbon decomposition in water".JOURNAL OF HAZARDOUS MATERIALS 469(2024). |
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