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DOI10.1016/j.cherd.2023.12.023
Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment
Ahmadi, Ali Reza; Rahimpour, Mohammad Reza; Farsi, Mohammad
发表日期2024
ISSN0263-8762
EISSN1744-3563
起始页码202
卷号202
英文摘要Carbon capture and carbon reuse in the chemical plants is one of the attractive prospective approaches to decrease the concerns about global warming and climate change. In the present study, is focused on the synthesis gas production from carbon dioxide in a methanol synthesis plant. In this regard, two methanol processes are proposed based on CO2 separation, recycling, and reforming. In the first scenario, CO2 is separated and recycled to the conventional reformer, while the process is equipped by a CO2 separation unit and dry methane reformer in the second scenario. The proposed processes are simulated and a sensitivity analysis is performed to investigated the effect of inputs on methanol productivity and carbon conversion. The operational parameters of proposed processes are optimized to enhance methanol productivity and CO2 conversion. Then, the processes are compared from energy efficiency, carbon efficiency, CO2 emission rate and methanol productivity viewpoints. The results showed that, in the second proposed scenario, methanol production rate approach to 5367 tons per day in comparison to 5030 tons per day for industrial unit. In addition, modification of conventional methanol process based on the second scenario could decrease CO2 emission rate about 56 tons per day.
英文关键词Process Simulation; MeOH; Carbon capture and recycling; Dry reforming
语种英语
WOS研究方向Engineering
WOS类目Engineering, Chemical
WOS记录号WOS:001164560100001
来源期刊CHEMICAL ENGINEERING RESEARCH & DESIGN
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/294551
作者单位Shiraz University
推荐引用方式
GB/T 7714
Ahmadi, Ali Reza,Rahimpour, Mohammad Reza,Farsi, Mohammad. Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment[J],2024,202.
APA Ahmadi, Ali Reza,Rahimpour, Mohammad Reza,&Farsi, Mohammad.(2024).Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment.CHEMICAL ENGINEERING RESEARCH & DESIGN,202.
MLA Ahmadi, Ali Reza,et al."Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment".CHEMICAL ENGINEERING RESEARCH & DESIGN 202(2024).
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