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DOI | 10.1016/j.cherd.2023.12.023 |
Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment | |
Ahmadi, Ali Reza; Rahimpour, Mohammad Reza; Farsi, Mohammad | |
发表日期 | 2024 |
ISSN | 0263-8762 |
EISSN | 1744-3563 |
起始页码 | 202 |
卷号 | 202 |
英文摘要 | Carbon capture and carbon reuse in the chemical plants is one of the attractive prospective approaches to decrease the concerns about global warming and climate change. In the present study, is focused on the synthesis gas production from carbon dioxide in a methanol synthesis plant. In this regard, two methanol processes are proposed based on CO2 separation, recycling, and reforming. In the first scenario, CO2 is separated and recycled to the conventional reformer, while the process is equipped by a CO2 separation unit and dry methane reformer in the second scenario. The proposed processes are simulated and a sensitivity analysis is performed to investigated the effect of inputs on methanol productivity and carbon conversion. The operational parameters of proposed processes are optimized to enhance methanol productivity and CO2 conversion. Then, the processes are compared from energy efficiency, carbon efficiency, CO2 emission rate and methanol productivity viewpoints. The results showed that, in the second proposed scenario, methanol production rate approach to 5367 tons per day in comparison to 5030 tons per day for industrial unit. In addition, modification of conventional methanol process based on the second scenario could decrease CO2 emission rate about 56 tons per day. |
英文关键词 | Process Simulation; MeOH; Carbon capture and recycling; Dry reforming |
语种 | 英语 |
WOS研究方向 | Engineering |
WOS类目 | Engineering, Chemical |
WOS记录号 | WOS:001164560100001 |
来源期刊 | CHEMICAL ENGINEERING RESEARCH & DESIGN
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/294551 |
作者单位 | Shiraz University |
推荐引用方式 GB/T 7714 | Ahmadi, Ali Reza,Rahimpour, Mohammad Reza,Farsi, Mohammad. Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment[J],2024,202. |
APA | Ahmadi, Ali Reza,Rahimpour, Mohammad Reza,&Farsi, Mohammad.(2024).Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment.CHEMICAL ENGINEERING RESEARCH & DESIGN,202. |
MLA | Ahmadi, Ali Reza,et al."Efficient recycling and conversion of CO2 to methanol: Process design and environmental assessment".CHEMICAL ENGINEERING RESEARCH & DESIGN 202(2024). |
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