气候变化领域集成服务门户(CCPortal): Separation of CO2/N2 onto Shaped MOF MIL-160(Al) Using the Pressure Swing Adsorption Process for Post-combustion Application

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DOI	10.1021/acs.iecr.4c00611
	Separation of CO2/N2 onto Shaped MOF MIL-160(Al) Using the Pressure Swing Adsorption Process for Post-combustion Application
	Karimi, Mohsen; Siqueira, Rafael M.; Rodrigues, Alirio E.; Nouar, Farid; Silva, Jose A. C.; Serre, Christian; Ferreira, Alexandre F. P.
发表日期	2024
ISSN	0888-5885
EISSN	1520-5045
起始页码	63
结束页码	19
卷号	63 期号:19
英文摘要	Adsorption processes have already been considered as an appealing technology for carbon capture and climate change mitigation. Accordingly, this work investigated the capacity of shaped MIL-160(Al) as a water stable bioderived Al dicarboxylate microporous metal-organic framework for separation of carbon dioxide and nitrogen concerning postcombustion application. First, breakthrough experiments of carbon dioxide and nitrogen were accomplished at 313 K and 4.0 bar. Then, a set of equations/relations were considered to model the dynamic fixed-bed tests, in which the outcomes proved the capacity of the developed model for such a purpose. Next, a pressure swing adsorption (PSA) process with five steps, including pressurization, feed, rinse, blowdown, and purge, was planned and validated using performed experiments in a laboratory-scale PSA setup. In the end, an industrial PSA process was designed to attain a better grasp of the capacity of MIL-160(Al) for postcombustion application. The results indicated an exciting potential of this adsorbent for postcombustion carbon capture, with the purity and recovery of carbon dioxide around 67.3 and 99.1%, respectively.
语种	英语
WOS研究方向	Engineering
WOS类目	Engineering, Chemical
WOS记录号	WOS:001226098200001
来源期刊	INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/293786
作者单位	Universidade do Porto; Universidade do Porto; Universite PSL; Ecole Normale Superieure (ENS); Ecole Superieure de Physique et de Chimie Industrielles de la Ville de Paris (ESPCI); Centre National de la Recherche Scientifique (CNRS); Instituto Politecnico de Braganca; Instituto Politecnico de Braganca
推荐引用方式 GB/T 7714	Karimi, Mohsen,Siqueira, Rafael M.,Rodrigues, Alirio E.,et al. Separation of CO2/N2 onto Shaped MOF MIL-160(Al) Using the Pressure Swing Adsorption Process for Post-combustion Application[J],2024,63(19).
APA	Karimi, Mohsen.,Siqueira, Rafael M..,Rodrigues, Alirio E..,Nouar, Farid.,Silva, Jose A. C..,...&Ferreira, Alexandre F. P..(2024).Separation of CO2/N2 onto Shaped MOF MIL-160(Al) Using the Pressure Swing Adsorption Process for Post-combustion Application.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,63(19).
MLA	Karimi, Mohsen,et al."Separation of CO2/N2 onto Shaped MOF MIL-160(Al) Using the Pressure Swing Adsorption Process for Post-combustion Application".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 63.19(2024).