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DOI | 10.1002/apj.3058 |
K2CO3 on porous supports for moisture-swing CO2 capture from ambient air | |
Zheng, Shiqiang; Cheng, Xinyue; Zhou, Wenjia; Wang, Tong; Zhu, Liangliang; Xiao, Hang; Chen, Xi | |
发表日期 | 2024 |
ISSN | 1932-2135 |
EISSN | 1932-2143 |
起始页码 | 19 |
结束页码 | 3 |
卷号 | 19期号:3 |
英文摘要 | Direct air capture (DAC) of CO2 is an important technology to mitigate mobile carbon emissions, reduce atmospheric CO2 concentration, and cope with climate change. Moisture-swing adsorption is regarded as one of the most promising technologies in DAC due to its low energy consumption and ease of operation. In this work, a cheap and easily available moisture-swing adsorbent of potassium carbonate loaded on porous supports (i.e., activated carbon, magnesium oxide, and zeolite) was prepared for CO2 capture from ambient air. The composite adsorbent of potassium carbonate on activated carbon showed the best performance with a DAC capacity of 0.562 mmol/g at 25 degrees C and 5% relative humidity. The effects of temperature, relative humidity, and CO2 concentration on the adsorption performance were investigated systematically, as well as the cyclic DAC performance. In 50 adsorption-desorption cycles, the adsorption capacity of the composite adsorbent decreased by similar to 40% due to potassium carbonate leaching loss during water evaporation but can be fully recovered simply by re-impregnating with potassium carbonate again. |
英文关键词 | activated carbon; direct air capture; moisture-swing; potassium carbonate |
语种 | 英语 |
WOS研究方向 | Engineering |
WOS类目 | Engineering, Chemical |
WOS记录号 | WOS:001186249500001 |
来源期刊 | ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/293360 |
作者单位 | Northwest University Xi'an; Lingnan University |
推荐引用方式 GB/T 7714 | Zheng, Shiqiang,Cheng, Xinyue,Zhou, Wenjia,et al. K2CO3 on porous supports for moisture-swing CO2 capture from ambient air[J],2024,19(3). |
APA | Zheng, Shiqiang.,Cheng, Xinyue.,Zhou, Wenjia.,Wang, Tong.,Zhu, Liangliang.,...&Chen, Xi.(2024).K2CO3 on porous supports for moisture-swing CO2 capture from ambient air.ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING,19(3). |
MLA | Zheng, Shiqiang,et al."K2CO3 on porous supports for moisture-swing CO2 capture from ambient air".ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING 19.3(2024). |
条目包含的文件 | 条目无相关文件。 |
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