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DOI10.1002/apj.3058
K2CO3 on porous supports for moisture-swing CO2 capture from ambient air
发表日期2024
ISSN1932-2135
EISSN1932-2143
起始页码19
结束页码3
卷号19期号:3
英文摘要Direct air capture (DAC) of CO2 is an important technology to mitigate mobile carbon emissions, reduce atmospheric CO2 concentration, and cope with climate change. Moisture-swing adsorption is regarded as one of the most promising technologies in DAC due to its low energy consumption and ease of operation. In this work, a cheap and easily available moisture-swing adsorbent of potassium carbonate loaded on porous supports (i.e., activated carbon, magnesium oxide, and zeolite) was prepared for CO2 capture from ambient air. The composite adsorbent of potassium carbonate on activated carbon showed the best performance with a DAC capacity of 0.562 mmol/g at 25 degrees C and 5% relative humidity. The effects of temperature, relative humidity, and CO2 concentration on the adsorption performance were investigated systematically, as well as the cyclic DAC performance. In 50 adsorption-desorption cycles, the adsorption capacity of the composite adsorbent decreased by similar to 40% due to potassium carbonate leaching loss during water evaporation but can be fully recovered simply by re-impregnating with potassium carbonate again.
英文关键词activated carbon; direct air capture; moisture-swing; potassium carbonate
语种英语
WOS研究方向Engineering
WOS类目Engineering, Chemical
WOS记录号WOS:001186249500001
来源期刊ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/293359
作者单位Northwest University Xi'an; Lingnan University
推荐引用方式
GB/T 7714
. K2CO3 on porous supports for moisture-swing CO2 capture from ambient air[J],2024,19(3).
APA (2024).K2CO3 on porous supports for moisture-swing CO2 capture from ambient air.ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING,19(3).
MLA "K2CO3 on porous supports for moisture-swing CO2 capture from ambient air".ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING 19.3(2024).
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