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DOI | 10.1021/acs.est.3c09516 |
Estimate Gaps of Montreal Protocol-Regulated Potent Greenhouse Gas HFC-152a Emissions in China Have Been Explained | |
Du, Qianna; Li, Bowei; Ma, Mengyue; Yao, Bo; Fang, Xuekun | |
发表日期 | 2024 |
ISSN | 0013-936X |
EISSN | 1520-5851 |
起始页码 | 58 |
结束页码 | 13 |
卷号 | 58期号:13 |
英文摘要 | 1,1-Difluoroethane (HFC-152a) is a hydrofluorocarbon regulated by the Montreal Protocol, and its emissions in China are of concern as China will regulate HFC-152a in 2024. However, no observation-inferred top-down estimates were undertaken after 2017, and substantial gaps existed among previous estimates of China's HFC-152a emissions. Using the atmospheric observations and inverse modeling, this study reveals China's HFC-152a emissions of 9.4 +/- 1.7 Gg/yr (gigagrams per year), 10.6 +/- 1.8 Gg/yr, and 9.7 +/- 1.5 Gg/yr in 2018, 2019, and 2020, respectively. In addition, we display an overall increasing trend during 2011-2020, which is in contrast to the decreasing and steady trend reported by the Emission Database for Global Atmospheric Research (EDGAR) and the Chinese government, respectively. Subsequently, we establish a comprehensive bottom-up emission inventory matching with top-down estimates and thus succeed in explaining the gaps among previous estimates. Furthermore, the contribution of China's emissions to global HFC-152a emission growth increased from 15% during 2001-2010 to >100% during 2011-2020. An emission projection based on our improved inventory shows that the Kigali Amendment (KA) would assist in avoiding 1535.6-4710.6 Gg (251.8-772.5 Tg CO2-eq) HFC-152a emissions during 2024-2100. Our findings indicate relatively accurate China's HFC-152a emissions and provide scientific support for addressing climate change and implementing the KA. |
英文关键词 | HFC-152a (CH3CHF2); emission gap; China; inverse modeling; climate change; Montreal Protocol |
语种 | 英语 |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
WOS类目 | Engineering, Environmental ; Environmental Sciences |
WOS记录号 | WOS:001189154200001 |
来源期刊 | ENVIRONMENTAL SCIENCE & TECHNOLOGY |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/289207 |
作者单位 | Zhejiang University; Fudan University; Fudan University; Massachusetts Institute of Technology (MIT); Peking University |
推荐引用方式 GB/T 7714 | Du, Qianna,Li, Bowei,Ma, Mengyue,et al. Estimate Gaps of Montreal Protocol-Regulated Potent Greenhouse Gas HFC-152a Emissions in China Have Been Explained[J],2024,58(13). |
APA | Du, Qianna,Li, Bowei,Ma, Mengyue,Yao, Bo,&Fang, Xuekun.(2024).Estimate Gaps of Montreal Protocol-Regulated Potent Greenhouse Gas HFC-152a Emissions in China Have Been Explained.ENVIRONMENTAL SCIENCE & TECHNOLOGY,58(13). |
MLA | Du, Qianna,et al."Estimate Gaps of Montreal Protocol-Regulated Potent Greenhouse Gas HFC-152a Emissions in China Have Been Explained".ENVIRONMENTAL SCIENCE & TECHNOLOGY 58.13(2024). |
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