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DOI10.1007/s11368-023-03462-6
Contamination characteristics, source analysis, and spatial prediction of soil heavy metal concentrations on the Qinghai-Tibet Plateau
Du, Haolin; Wang, Jinsong; Wang, Ying; Yao, Yubi; Liu, Xiaoyun; Zhou, Yue
发表日期2023
ISSN1439-0108
EISSN1614-7480
起始页码2202
结束页码2215
卷号23期号:5
英文摘要PurposeSoil heavy metal distribution is a key issue in environmental and health research. In recent years, an increasing number of anthropogenic disturbances have been identified on the Qinghai-Tibetan Plateau, leading to increased heavy metal contamination of soils. Therefore, this study investigated the distribution, sources, ecological risk, and prediction of heavy metals in soils on the Qinghai-Tibetan Plateau.Material and methodsHere, for each of the seven heavy metals (i.e., Cr, Ni, Cu, Zn, As, Cd, and Pb) investigated in the soil of the Qinghai-Tibet Plateau, we collected soil concentration values from the literature and carried out field sampling to generate new data. We then assessed the pollution characteristics and sources of soil heavy metals on the Qinghai-Tibet Plateau using geostatistics, positive matrix factorization model (PMF), disjunctive kriging, and mapped the pollution risk probability distribution of each heavy metal element.Results and discussionSpatial autocorrelation was found for all seven heavy metals in the soils. Under different land-use types, the average concentrations of Cr, As, and Cd were highest in the water areas; Ni levels were highest in woodland; and Cu, Zn, and Pb concentrations were highest in residential, industrial, and mining lands. Using analysis by the PMF model and correlation analysis, four heavy metal sources were identified, including industrial sources and atmospheric deposition (Cd), traffic emissions (Cr, Zn, and Zn), natural sources (Ni and As), and mining activities (Cr and Pb). The pollution risk probabilities of Cr, Ni, Cu, Zn, As, and Pb were low in most areas of the Qinghai-Tibet Plateau, whereas the pollution risk probability of Cd was high over 29% of the area of the Qinghai-Tibet Plateau.ConclusionThe results highlighted no potential contamination for Cr, local potential contamination for Ni, Cu, Zn, As and Pb, while Cd exhibits more extensive contamination in the soils of the Qinghai-Tibet Plateau. Cd reduction should therefore be considered an important component of the strategy, policy, and action plan for soil pollution management on the Qinghai-Tibet Plateau.
关键词Qinghai-Tibet PlateauSoilHeavy metalsGeostatistical analysisSourcesDisjunctive kriging
英文关键词POSITIVE MATRIX FACTORIZATION; HEALTH-RISK ASSESSMENT; SOURCE APPORTIONMENT; AGRICULTURAL SOIL; GLOBAL POLLUTION; SEDIMENTS; IDENTIFICATION; VARIABILITY; ENRICHMENT; WATER
WOS研究方向Environmental Sciences ; Soil Science
WOS记录号WOS:000946841800002
来源期刊JOURNAL OF SOILS AND SEDIMENTS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/282623
作者单位China Meteorological Administration; China Meteorological Administration; China Meteorological Administration
推荐引用方式
GB/T 7714
Du, Haolin,Wang, Jinsong,Wang, Ying,et al. Contamination characteristics, source analysis, and spatial prediction of soil heavy metal concentrations on the Qinghai-Tibet Plateau[J],2023,23(5).
APA Du, Haolin,Wang, Jinsong,Wang, Ying,Yao, Yubi,Liu, Xiaoyun,&Zhou, Yue.(2023).Contamination characteristics, source analysis, and spatial prediction of soil heavy metal concentrations on the Qinghai-Tibet Plateau.JOURNAL OF SOILS AND SEDIMENTS,23(5).
MLA Du, Haolin,et al."Contamination characteristics, source analysis, and spatial prediction of soil heavy metal concentrations on the Qinghai-Tibet Plateau".JOURNAL OF SOILS AND SEDIMENTS 23.5(2023).
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