气候变化领域集成服务门户(CCPortal): Rational Design of Better Hydrogen Evolution Electrocatalysts for Water Splitting: A Review

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DOI	10.1002/advs.202200307
	Rational Design of Better Hydrogen Evolution Electrocatalysts for Water Splitting: A Review
	Liu, Fan; Shi, Chengxiang; Guo, Xiaolei; He, Zexing; Pan, Lun; Huang, Zhen-Feng; Zhang, Xiangwen; Zou, Ji-Jun
发表日期	2022
EISSN	2198-3844
卷号	9 期号:18
英文摘要	The excessive dependence on fossil fuels contributes to the majority of CO2 emissions, influencing on the climate change. One promising alternative to fossil fuels is green hydrogen, which can be produced through water electrolysis from renewable electricity. However, the variety and complexity of hydrogen evolution electrocatalysts currently studied increases the difficulty in the integration of catalytic theory, catalyst design and preparation, and characterization methods. Herein, this review first highlights design principles for hydrogen evolution reaction (HER) electrocatalysts, presenting the thermodynamics, kinetics, and related electronic and structural descriptors for HER. Second, the reasonable design, preparation, mechanistic understanding, and performance enhancement of electrocatalysts are deeply discussed based on intrinsic and extrinsic effects. Third, recent advancements in the electrocatalytic water splitting technology are further discussed briefly. Finally, the challenges and perspectives of the development of highly efficient hydrogen evolution electrocatalysts for water splitting are proposed.
英文关键词	catalyst design; extrinsic effects; hydrogen evolution reaction; intrinsic effects; water-splitting technology
语种	英语
WOS研究方向	Chemistry, Multidisciplinary ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS类目	Science Citation Index Expanded (SCI-EXPANDED)
WOS记录号	WOS:000783221300001
来源期刊	ADVANCED SCIENCE
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/280833
作者单位	Tianjin University; Tianjin University
推荐引用方式 GB/T 7714	Liu, Fan,Shi, Chengxiang,Guo, Xiaolei,et al. Rational Design of Better Hydrogen Evolution Electrocatalysts for Water Splitting: A Review[J],2022,9(18).
APA	Liu, Fan.,Shi, Chengxiang.,Guo, Xiaolei.,He, Zexing.,Pan, Lun.,...&Zou, Ji-Jun.(2022).Rational Design of Better Hydrogen Evolution Electrocatalysts for Water Splitting: A Review.ADVANCED SCIENCE,9(18).
MLA	Liu, Fan,et al."Rational Design of Better Hydrogen Evolution Electrocatalysts for Water Splitting: A Review".ADVANCED SCIENCE 9.18(2022).