气候变化领域集成服务门户(CCPortal): Aerosol-stratocumulus interactions: towards a better process understanding using closures between observations and large eddy simulations

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DOI	10.5194/acp-22-12417-2022
	Aerosol-stratocumulus interactions: towards a better process understanding using closures between observations and large eddy simulations
	Calderon, Silvia M.; Tonttila, Juha; Buchholz, Angela; Joutsensaari, Jorma; Komppula, Mika; Leskinen, Ari; Hao, Liqing; Moisseev, Dmitri; Pullinen, Iida; Tiitta, Petri; Xu, Jian; Virtanen, Annele; Kokkola, Harri; Romakkaniemi, Sami
发表日期	2022
ISSN	1680-7316
EISSN	1680-7324
起始页码	12417
结束页码	12441
卷号	22 期号:18 页码:25
英文摘要	We carried out a closure study of aerosol-cloud interactions during stratocumulus formation using a large eddy simulation model UCLALES-SALSA (University of California Los Angeles large eddy simulation model-sectional aerosol module for large applications) and observations from the 2020 cloud sampling campaign at Puijo SMEAR IV (Station for Measuring Ecosystem-Atmosphere Relations) in Kuopio, Finland. The unique observational setup combining in situ and cloud remote sensing measurements allowed a closer look into the aerosol size-composition dependence of droplet activation and droplet growth in turbulent boundary layer driven by surface forcing and radiative cooling. UCLALES-SALSA uses spectral bin microphysics for aerosols and hydrometeors, and incorporates a full description of their interactions into the turbulent-convective radiation-dynamical model of stratocumulus. Based on our results, the model successfully described the probability distribution of updraught velocities and consequently the size dependency of aerosol activation into cloud droplets, and further recreated the size distributions for both interstitial aerosol and cloud droplets. This is the first time such a detailed closure is achieved not only accounting for activation of cloud droplets in different updraughts, but also accounting for processes evaporating droplets and drizzle production through coagulation-coalescence. We studied two cases of cloud formation, one diurnal (24 September 2020) and one nocturnal (31 October 2020), with high and low aerosol loadings, respectively. Aerosol number concentrations differ more than 1 order of magnitude between cases and therefore, lead to cloud droplet number concentration (CDNC) values which range from less than 100 cm(-3) up to 1000 cm(-3). Different aerosol loadings affected supersaturation at the cloud base, and thus the size of aerosol particles activating to cloud droplets. Due to higher CDNC, the mean size of cloud droplets in the diurnal high aerosol case was lower. Thus, droplet evaporation in downdraughts affected more the observed CDNC at Puijo altitude compared to the low aerosol case. In addition, in the low aerosol case, the presence of large aerosol particles in the accumulation mode played a significant role in the droplet spectrum evolution as it promoted the drizzle formation through collision and coalescence processes. Also, during the event, the formation of ice particles was observed due to subzero temperature at the cloud top. Although the modelled number concentration of ice hydrometeors was too low to be directly measured, the retrieval of hydrometeor sedimentation velocities with cloud radar allowed us to assess the realism of modelled ice particles. The studied cases are presented in detail and can be further used by the cloud modellers to test and validate their models in a well-characterized modelling setup. We also provide recommendations on how increasing amount of information on aerosol properties could improve the understanding of processes affecting cloud droplet number and liquid water content in stratiform clouds.
学科领域	Environmental Sciences; Meteorology & Atmospheric Sciences
语种	英语
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号	WOS:000856069300001
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/273919
作者单位	Finnish Meteorological Institute; University of Eastern Finland; University of Helsinki; Finnish Meteorological Institute; Helmholtz Association; Research Center Julich
推荐引用方式 GB/T 7714	Calderon, Silvia M.,Tonttila, Juha,Buchholz, Angela,et al. Aerosol-stratocumulus interactions: towards a better process understanding using closures between observations and large eddy simulations[J],2022,22(18):25.
APA	Calderon, Silvia M..,Tonttila, Juha.,Buchholz, Angela.,Joutsensaari, Jorma.,Komppula, Mika.,...&Romakkaniemi, Sami.(2022).Aerosol-stratocumulus interactions: towards a better process understanding using closures between observations and large eddy simulations.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(18),25.
MLA	Calderon, Silvia M.,et al."Aerosol-stratocumulus interactions: towards a better process understanding using closures between observations and large eddy simulations".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.18(2022):25.