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DOI10.5194/acp-23-2557-2023
Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions
Huang, Yue; Kok, Jasper F.; Saito, Masanori; Munoz, Olga
发表日期2023
ISSN1680-7316
EISSN1680-7324
起始页码2557
结束页码2577
卷号23期号:4页码:21
英文摘要Most global aerosol models approximate dust as spherical particles, whereas most remote sensing retrieval algorithms approximate dust as spheroidal particles with a shape distribution that conflicts with mea-surements. These inconsistent and inaccurate shape assumptions generate biases in dust single-scattering proper-ties. Here, we obtain dust single-scattering properties by approximating dust as triaxial ellipsoidal particles with observationally constrained shape distributions. We find that, relative to the ellipsoidal dust optics obtained here, the spherical dust optics used in most aerosol models underestimate dust single-scattering albedo, mass extinc-tion efficiency, and asymmetry parameter for almost all dust sizes in both the shortwave and longwave spectra. We further find that the ellipsoidal dust optics are in substantially better agreement with observations of the scattering matrix and linear depolarization ratio than the spheroidal dust optics used in most retrieval algorithms. However, relative to observations, the ellipsoidal dust optics overestimate the lidar ratio by underestimating the backscattering intensity by a factor of similar to 2. This occurs largely because the computational method used to simulate ellipsoidal dust optics (i.e., the improved geometric optics method) underestimates the backscattering intensity by a factor of similar to 2 relative to other computational methods (e.g., the physical geometric optics method). We conclude that the ellipsoidal dust optics with observationally constrained shape distributions can help im-prove global aerosol models and possibly remote sensing retrieval algorithms that do not use the backscattering signal.
学科领域Environmental Sciences; Meteorology & Atmospheric Sciences
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000937273400001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/273904
作者单位University of California System; University of California Los Angeles; Texas A&M University System; Texas A&M University College Station; Consejo Superior de Investigaciones Cientificas (CSIC); CSIC - Instituto de Astrofisica de Andalucia (IAA); Columbia University; National Aeronautics & Space Administration (NASA)
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Huang, Yue,Kok, Jasper F.,Saito, Masanori,et al. Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions[J],2023,23(4):21.
APA Huang, Yue,Kok, Jasper F.,Saito, Masanori,&Munoz, Olga.(2023).Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions.ATMOSPHERIC CHEMISTRY AND PHYSICS,23(4),21.
MLA Huang, Yue,et al."Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions".ATMOSPHERIC CHEMISTRY AND PHYSICS 23.4(2023):21.
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