气候变化领域集成服务门户(CCPortal): Stable water isotope signals in tropical ice clouds in the West African monsoon simulated with a regional convection-permitting model

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DOI	10.5194/acp-22-8863-2022
	Stable water isotope signals in tropical ice clouds in the West African monsoon simulated with a regional convection-permitting model
	de Vries, Andries Jan; Aemisegger, Franziska; Pfahl, Stephan; Wernli, Heini
发表日期	2022
ISSN	1680-7316
EISSN	1680-7324
起始页码	8863
结束页码	8895
卷号	22 期号:13 页码:33
英文摘要	Tropical ice clouds have an important influence on the Earth's radiative balance. They often form as a result of tropical deep convection, which strongly affects the water budget of the tropical tropopause layer. Ice cloud formation involves complex interactions on various scales. These processes are not yet fully understood and lead to large uncertainties in climate projections. In this study, we investigate the formation of tropical ice clouds related to deep convection in the West African monsoon, using stable water isotopes as tracers of moist atmospheric processes. We perform convection-permitting simulations with the regional Consortium for Small-Scale Modelling isotope-enabled (COSMOiso) model for the period from June to July 2016. First, we evaluate our model simulations using space-borne observations of mid-tropospheric water vapour isotopes, monthly station data of precipitation isotopes, and satellite-based precipitation estimates. Next, we explore the isotope signatures of tropical deep convection in atmospheric water vapour and ice based on a case study of a mesoscale convective system (MCS) and a statistical analysis of a 1-month period. The following five key processes related to tropical ice clouds can be distinguished based on isotope information: (1) convective lofting of enriched ice into the upper troposphere, (2) cirrus clouds that form in situ from ambient vapour under equilibrium fractionation, (3) sedimentation and sublimation of ice in the mixed-phase cloud layer in the vicinity of convective systems and underneath cirrus shields, (4) sublimation of ice in convective downdraughts that enriches the environmental vapour, and (5) the freezing of liquid water just above the 0 degrees C isotherm in convective updraughts. Importantly, we note large variations in the isotopic composition of water vapour in the upper troposphere and lower tropical tropopause layer, ranging from below -800 parts per thousand to over -400 parts per thousand, which are strongly related to vertical motion and the moist processes that take place in convective updraughts and downdraughts. In convective updraughts, the vapour is depleted by the preferential condensation and deposition of heavy isotopes, whereas the non-fractionating sublimation of ice in convective downdraughts enriches the environmental vapour. An opposite vapour isotope signature emerges in thin-cirrus cloud regions where the direct transport of enriched (depleted) vapour prevails in large-scale ascent (descent). Overall, this study demonstrates that isotopes can serve as useful tracers to disentangle the role of different processes in the West African monsoon water cycle, including convective transport, the formation of ice clouds, and their impact on the tropical tropopause layer.
学科领域	Environmental Sciences; Meteorology & Atmospheric Sciences
语种	英语
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号	WOS:000822752300001
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/273710
作者单位	Swiss Federal Institutes of Technology Domain; ETH Zurich; Free University of Berlin
推荐引用方式 GB/T 7714	de Vries, Andries Jan,Aemisegger, Franziska,Pfahl, Stephan,et al. Stable water isotope signals in tropical ice clouds in the West African monsoon simulated with a regional convection-permitting model[J],2022,22(13):33.
APA	de Vries, Andries Jan,Aemisegger, Franziska,Pfahl, Stephan,&Wernli, Heini.(2022).Stable water isotope signals in tropical ice clouds in the West African monsoon simulated with a regional convection-permitting model.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(13),33.
MLA	de Vries, Andries Jan,et al."Stable water isotope signals in tropical ice clouds in the West African monsoon simulated with a regional convection-permitting model".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.13(2022):33.