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DOI10.5194/acp-22-9663-2022
The ice-nucleating activity of African mineral dust in the Caribbean boundary layer
Harrison, Alexander D.; O'Sullivan, Daniel; Adams, Michael P.; Porter, Grace C. E.; Blades, Edmund; Brathwaite, Cherise; Chewitt-Lucas, Rebecca; Gaston, Cassandra; Hawker, Rachel; Krueger, Ovid O.; Neve, Leslie; Poehlker, Mira L.; Poehlker, Christopher; Poeschl, Ulrich; Sanchez-Marroquin, Alberto; Sealy, Andrea; Sealy, Peter; Tarn, Mark D.; Whitehall, Shanice; McQuaid, James B.; Carslaw, Kenneth S.; Prospero, Joseph M.; Murray, Benjamin J.
发表日期2022
ISSN1680-7316
EISSN1680-7324
起始页码9663
结束页码9680
卷号22期号:14页码:18
英文摘要African mineral dust is transported many thousands of kilometres from its source regions, and, because of its ability to nucleate ice, it plays a major role in cloud glaciation around the globe. The ice-nucleating activity of desert dust is influenced by its mineralogy, which varies substantially between source regions and across particle sizes. However, in models it is often assumed that the activity (expressed as active sites per unit surface area as a function of temperature) of atmospheric mineral dust is the same everywhere on the globe. Here, we find that the ice-nucleating activity of African desert dust sampled in the summertime marine boundary layer of Barbados (July and August 2017) is substantially lower than parameterizations based on soil from specific locations in the Sahara or dust sedimented from dust storms. We conclude that the activity of dust in Barbados' boundary layer is primarily defined by the low K-feldspar content of the dust, which is around 1 %. We propose that the dust we sampled in the Caribbean was from a region in western Africa (in and around the Sahel in Mauritania and Mali), which has a much lower feldspar content than other African sources across the Sahara and Sahel.
学科领域Environmental Sciences; Meteorology & Atmospheric Sciences
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000832642700001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/273640
作者单位University of Leeds; University of Miami; Max Planck Society; Leibniz Institut fur Tropospharenforschung (TROPOS); Leipzig University
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Harrison, Alexander D.,O'Sullivan, Daniel,Adams, Michael P.,et al. The ice-nucleating activity of African mineral dust in the Caribbean boundary layer[J],2022,22(14):18.
APA Harrison, Alexander D..,O'Sullivan, Daniel.,Adams, Michael P..,Porter, Grace C. E..,Blades, Edmund.,...&Murray, Benjamin J..(2022).The ice-nucleating activity of African mineral dust in the Caribbean boundary layer.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(14),18.
MLA Harrison, Alexander D.,et al."The ice-nucleating activity of African mineral dust in the Caribbean boundary layer".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.14(2022):18.
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