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DOI10.5194/acp-22-11125-2022
Bayesian assessment of chlorofluorocarbon (CFC), hydrochlorofluorocarbon (HCFC) and halon banks suggest large reservoirs still present in old equipment
Lickley, Megan Jeramaz; Daniel, John S.; Fleming, Eric L.; Reimann, Stefan; Solomon, Susan
发表日期2022
ISSN1680-7316
EISSN1680-7324
起始页码11125
结束页码11136
卷号22期号:17页码:12
英文摘要Halocarbons contained in equipment such as air conditioners, fire extinguishers, and foams continue to be emitted after production has ceased. These banks within equipment and applications are thus potential sources of future emissions, and must be carefully accounted for in order to differentiate nascent and potentially illegal production from legal banked emissions. Here, we build on a probabilistic Bayesian model, previously developed to quantify chlorofluorocarbon (CFC-11, CFC-12, and CFC-113) banks and their emissions. We extend this model to a suite of banked chemicals regulated under the Montreal Protocol (hydrochlorofluorocarbon, HCFC-22, HCFC-141b, and HCFC-142b, halon 1211 and halon 1301, and CFC-114 and CFC-115) along with CFC-11, CFC-12, and CFC-113 in order to quantify a fuller range of ozone-depleting substance (ODS) banks by chemical and equipment type. We show that if atmospheric lifetime and prior assumptions are accurate, banks are most likely larger than previous international assessments suggest, and that total production has probably been higher than reported. We identify that banks of greatest climate-relevance, as determined by global warming potential weighting, are largely concentrated in CFC-11 foams and CFC-12 and HCFC-22 non-hermetic refrigeration. Halons, CFC-11, and CFC-12 banks dominate the banks weighted by ozone depletion potential (ODP). Thus, we identify and quantify the uncertainties in substantial banks whose future emissions will contribute to future global warming and delay ozone-hole recovery if left unrecovered.
学科领域Environmental Sciences; Meteorology & Atmospheric Sciences
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000848180300001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/273609
作者单位Massachusetts Institute of Technology (MIT); National Aeronautics & Space Administration (NASA); NASA Goddard Space Flight Center; Science Systems and Applications Inc; Swiss Federal Institutes of Technology Domain; Swiss Federal Laboratories for Materials Science & Technology (EMPA)
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Lickley, Megan Jeramaz,Daniel, John S.,Fleming, Eric L.,et al. Bayesian assessment of chlorofluorocarbon (CFC), hydrochlorofluorocarbon (HCFC) and halon banks suggest large reservoirs still present in old equipment[J],2022,22(17):12.
APA Lickley, Megan Jeramaz,Daniel, John S.,Fleming, Eric L.,Reimann, Stefan,&Solomon, Susan.(2022).Bayesian assessment of chlorofluorocarbon (CFC), hydrochlorofluorocarbon (HCFC) and halon banks suggest large reservoirs still present in old equipment.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(17),12.
MLA Lickley, Megan Jeramaz,et al."Bayesian assessment of chlorofluorocarbon (CFC), hydrochlorofluorocarbon (HCFC) and halon banks suggest large reservoirs still present in old equipment".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.17(2022):12.
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