气候变化领域集成服务门户(CCPortal): Overview: On the transport and transformation of pollutants in the outflow of major population centres - observational data from the EMeRGe European intensive operational period in summer 2017

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DOI	10.5194/acp-22-5877-2022
	Overview: On the transport and transformation of pollutants in the outflow of major population centres - observational data from the EMeRGe European intensive operational period in summer 2017
	Andres Hernandez, M. Dolores; Hilboll, Andreas; Ziereis, Helmut; Foerster, Eric; Krueger, Ovid O.; Kaiser, Katharina; Schneider, Johannes; Barnaba, Francesca; Vrekoussis, Mihalis; Schmidt, Joerg; Huntrieser, Heidi; Blechschmidt, Anne-Marlene; George, Midhun; Nenakhov, Vladyslav; Harlass, Theresa; Holanda, Bruna A.; Wolf, Jennifer; Eirenschmalz, Lisa; Krebsbach, Marc; Poehlker, Mira L.; Kalisz Hedegaard, Anna B.; Mei, Linlu; Pfeilsticker, Klaus; Liu, Yangzhuoran; Koppmann, Ralf; Schlager, Hans; Bohn, Birger; Schumann, Ulrich; Richter, Andreas; Schreiner, Benjamin; Sauer, Daniel; Baumann, Robert; Mertens, Mariano; Joeckel, Patrick; Kilian, Markus; Stratmann, Greta; Poehlker, Christopher; Campanelli, Monica; Pandolfi, Marco; Sicard, Michael; Gomez-Amo, Jose L.; Pujadas, Manuel; Bigge, Katja; Kluge, Flora; Schwarz, Anja; Daskalakis, Nikos; Walter, David; Zahn, Andreas; Poeschl, Ulrich; Boenisch, Harald; Borrmann, Stephan; Platt, Ulrich; Burrows, John P.
发表日期	2022
ISSN	1680-7316
EISSN	1680-7324
起始页码	5877
结束页码	5924
卷号	22 期号:9 页码:48
英文摘要	Megacities and other major population centres (MPCs) worldwide are major sources of air pollution, both locally as well as downwind. The overall assessment and prediction of the impact of MPC pollution on tropospheric chemistry are challenging. The present work provides an overview of the highlights of a major new contribution to the understanding of this issue based on the data and analysis of the EMeRGe (Effect of Megacities on the transport and transformation of pollutants on the Regional to Global scales) international project. EMeRGe focuses on atmospheric chemistry, dynamics, and transport of local and regional pollution originating in MPCs. Airborne measurements, taking advantage of the long range capabilities of the High Altitude and LOng Range Research Aircraft (HALO, https://www.halo- spp.de, last access: 22 March 2022), are a central part of the project. The synergistic use and consistent interpretation of observational data sets of different spatial and temporal resolution (e.g. from ground-based networks, airborne campaigns, and satellite measurements) supported by modelling within EMeRGe provide unique insight to test the current understanding of MPC pollution outflows. In order to obtain an adequate set of measurements at different spatial scales, two field experiments were positioned in time and space to contrast situations when the photochemical transformation of plumes emerging from MPCs is large. These experiments were conducted in summer 2017 over Europe and in the inter-monsoon period over Asia in spring 2018. The intensive observational periods (IOPs) involved HALO airborne measurements of ozone and its precursors, volatile organic compounds, aerosol particles, and related species as well as coordinated ground-based ancillary observations at different sites. Perfluorocarbon (PFC) tracer releases and model forecasts supported the flight planning, the identification of pollution plumes, and the analysis of chemical transformations during transport. This paper describes the experimental deployment and scientific questions of the IOP in Europe. The MPC targets - London (United Kingdom; UK), the Benelux/Ruhr area (Belgium, the Netherlands, Luxembourg and Germany), Paris (France), Rome and the Po Valley (Italy), and Madrid and Barcelona (Spain) - were investigated during seven HALO research flights with an aircraft base in Germany for a total of 53 flight hours. An inflight comparison of HALO with the collaborating UK-airborne platform Facility for Airborne Atmospheric Measurements (FAAM) took place to assure accuracy and comparability of the instrumentation on board. Overall, EMeRGe unites measurements of near- and far-field emissions and hence deals with complex air masses of local and distant sources. Regional transport of several European MPC outflows was successfully identified and measured. Chemical processing of the MPC emissions was inferred from airborne observations of primary and secondary pollutants and the ratios between species having different chemical lifetimes. Photochemical processing of aerosol and secondary formation or organic acids was evident during the transport of MPC plumes. Urban plumes mix efficiently with natural sources as mineral dust and with biomass burning emissions from vegetation and forest fires. This confirms the importance of wildland fire emissions in Europe and indicates an important but discontinuous contribution to the European emission budget that might be of relevance in the design of efficient mitigation strategies. The present work provides an overview of the most salient results in the European context, with these being addressed in more detail within additional dedicated EMeRGe studies. The deployment and results obtained in Asia will be the subject of separate publications.
学科领域	Environmental Sciences; Meteorology & Atmospheric Sciences
语种	英语
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号	WOS:000790848000001
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/273561
作者单位	University of Bremen; University of Bremen; Helmholtz Association; German Aerospace Centre (DLR); Helmholtz Association; Karlsruhe Institute of Technology; Max Planck Society; Johannes Gutenberg University of Mainz; Max Planck Society; Consiglio Nazionale delle Ricerche (CNR); Istituto di Scienze dell'Atmosfera e del Clima (ISAC-CNR); Leipzig University; University of Wuppertal; Ruprecht Karls University Heidelberg; Helmholtz Association; Research Center Julich; Consejo Superior de Investigaciones Cientificas (CSIC); CSIC - Centro de Investigacion y Desarrollo Pascual Vila (CID-CSIC); CSIC - Instituto de Diagnostico Ambiental y Estudios del Agua (IDAEA); Universitat Politecnica de Catalunya; Institut d'Estudis Espacials de Catalunya (IEEC); Universitat Politecnica de Catalunya; University of Valencia; Centro de Investigaciones Energeticas, Medioambientales Tecnologicas; Helmholtz Association; German Aerospace Centre (DLR); Leibniz Institut fur Tropospharenforschung (TROPOS); Leipzig University; Helmholtz ...
推荐引用方式 GB/T 7714	Andres Hernandez, M. Dolores,Hilboll, Andreas,Ziereis, Helmut,et al. Overview: On the transport and transformation of pollutants in the outflow of major population centres - observational data from the EMeRGe European intensive operational period in summer 2017[J],2022,22(9):48.
APA	Andres Hernandez, M. Dolores.,Hilboll, Andreas.,Ziereis, Helmut.,Foerster, Eric.,Krueger, Ovid O..,...&Burrows, John P..(2022).Overview: On the transport and transformation of pollutants in the outflow of major population centres - observational data from the EMeRGe European intensive operational period in summer 2017.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(9),48.
MLA	Andres Hernandez, M. Dolores,et al."Overview: On the transport and transformation of pollutants in the outflow of major population centres - observational data from the EMeRGe European intensive operational period in summer 2017".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.9(2022):48.