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DOI10.5194/acp-22-12827-2022
Ozone, DNA-active UV radiation, and cloud changes for the near-global mean and at high latitudes due to enhanced greenhouse gas concentrations
Eleftheratos, Kostas; Kapsomenakis, John; Fountoulakis, Ilias; Zerefos, Christos S.; Jockel, Patrick; Dameris, Martin; Bais, Alkiviadis F.; Bernhard, Germar; Kouklaki, Dimitra; Tourpali, Kleareti; Stierle, Scott; Ben Liley, J.; Brogniez, Colette; Auriol, Frederique; Diemoz, Henri; Simic, Stana; Petropavlovskikh, Irina; Lakkala, Kaisa; Douvis, Kostas
发表日期2022
ISSN1680-7316
EISSN1680-7324
起始页码12827
结束页码12855
卷号22期号:19页码:29
英文摘要This study analyses the variability and trends of ultraviolet-B (UV-B, wavelength 280-320 nm) radiation that can cause DNA damage. The variability and trends caused by climate change due to enhanced greenhouse gas (GHG) concentrations. The analysis is based on DNA-active irradiance, total ozone, total cloud cover, and surface albedo calculations with the European Centre for Medium-Range Weather Forecasts - Hamburg (ECHAM)/Modular Earth Submodel System (MESSy) Atmospheric Chemistry (EMAC) chemistry-climate model (CCM) free-running simulations following the RCP 6.0 climate scenario for the period 1960-2100. The model output is evaluated with DNA-active irradiance ground-based measurements, satellite SBUV (v8.7) total-ozone measurements, and satellite MODerate-resolution Imaging Spectroradiometer (MODIS) Terra cloud cover data. The results show that the model reproduces the observed variability and change in total ozone, DNA-active irradiance, and cloud cover for the period 2000-2018 quite well according to the statistical comparisons. Between 50 degrees N-50 degrees S, the DNA-damaging UV radiation is expected to decrease until 2050 and to increase thereafter, as was shown previously by Eleftheratos et al. (2020). This change is associated with decreases in the model total cloud cover and negative trends in total ozone after about 2050 due to increasing GHGs. The new study confirms the previous work by adding more stations over low latitudes and mid-latitudes (13 instead of 5 stations). In addition, we include estimates from high-latitude stations with long-term measurements of UV irradiance (three stations in the northern high latitudes and four stations in the southern high latitudes greater than 55 degrees). In contrast to the predictions for 50 degrees N-50 degrees S, it is shown that DNA-active irradiance will continue to decrease after the year 2050 over high latitudes because of upward ozone trends. At latitudes poleward of 55 degrees N, we estimate that DNA-active irradiance will decrease by 8.2 % +/- 3.8 % from 2050 to 2100. Similarly, at latitudes poleward of 55 degrees S, DNA-active irradiance will decrease by 4.8 % +/- 2.9 % after 2050. The results for the high latitudes refer to the summer period and not to the seasons when ozone depletion occurs, i.e. in late winter and spring. The contributions of ozone, cloud, and albedo trends to the DNA-active irradiance trends are estimated and discussed.
学科领域Environmental Sciences; Meteorology & Atmospheric Sciences
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000864149000001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/273545
作者单位National & Kapodistrian University of Athens; Academy of Athens; Academy of Athens; Regional Environmental Protection Agency - Italy; Helmholtz Association; German Aerospace Centre (DLR); Aristotle University of Thessaloniki; National Institute of Water & Atmospheric Research (NIWA) - New Zealand; Centre National de la Recherche Scientifique (CNRS); CNRS - National Institute for Earth Sciences & Astronomy (INSU); Universite de Lille - ISITE; Universite de Lille; University of Natural Resources & Life Sciences, Vienna; University of Colorado System; University of Colorado Boulder; Finnish Meteorological Institute; Finnish Meteorological Institute
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Eleftheratos, Kostas,Kapsomenakis, John,Fountoulakis, Ilias,et al. Ozone, DNA-active UV radiation, and cloud changes for the near-global mean and at high latitudes due to enhanced greenhouse gas concentrations[J],2022,22(19):29.
APA Eleftheratos, Kostas.,Kapsomenakis, John.,Fountoulakis, Ilias.,Zerefos, Christos S..,Jockel, Patrick.,...&Douvis, Kostas.(2022).Ozone, DNA-active UV radiation, and cloud changes for the near-global mean and at high latitudes due to enhanced greenhouse gas concentrations.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(19),29.
MLA Eleftheratos, Kostas,et al."Ozone, DNA-active UV radiation, and cloud changes for the near-global mean and at high latitudes due to enhanced greenhouse gas concentrations".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.19(2022):29.
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