气候变化领域集成服务门户(CCPortal): Measurement report: Long-term changes in black carbon and aerosol optical properties from 2012 to 2020 in Beijing, China

CCPortal

DOI	10.5194/acp-22-561-2022
	Measurement report: Long-term changes in black carbon and aerosol optical properties from 2012 to 2020 in Beijing, China
	Sun, Jiaxing; Wang, Zhe; Zhou, Wei; Xie, Conghui; Wu, Cheng; Chen, Chun; Han, Tingting; Wang, Qingqing; Li, Zhijie; Li, Jie; Fu, Pingqing; Wang, Zifa; Sun, Yele
发表日期	2022
ISSN	1680-7316
EISSN	1680-7324
起始页码	561
结束页码	575
卷号	22 期号:1 页码:15
英文摘要	Atmospheric aerosols play an important role in the radiation balance of the earth-atmosphere system. However, our knowledge of the long-term changes in equivalent black carbon (eBC) and aerosol optical properties in China is very limited. Here we analyze the 9-year measurements of eBC and aerosol optical properties from 2012 to 2020 in Beijing, China. Our results showed large reductions in eBC by 71% from 6.25 +/- 5.73 mu g m(-3) in 2012 to 1.80 +/- 1.54 mu g m(-3) in 2020 and 47% decreases in the light extinction coefficient (b(ext), lambda = 630 nm) of fine particles due to the Clean Air Action Plan that was implemented in 2013. The seasonal and diurnal variations of eBC illustrated the most significant reductions in the fall and at nighttime, respectively. Delta eBC/Delta CO also showed an annual decrease from similar to 7 to 4 ng m(-3) ppbv(-1) and presented strong seasonal variations with high values in spring and fall, indicating that primary emissions in Beijing have changed significantly. As a response to the Clean Air Action Plan, single-scattering albedo (SSA) showed a considerable increase from 0.79 +/- 0.11 to 0.88 +/- 0.06, and mass extinction efficiency (MEE) increased from 3.2 to 3.8 m(2) g(-1). These results highlight the increasing importance of scattering aerosols in radiative forcing and a future challenge in visibility improvement due to enhanced MEE. Brown carbon (BrC) showed similar changes and seasonal variations to eBC during 2018-2020. However, we found a large increase of secondary BrC in the total BrC in most seasons, particularly in summer with the contribution up to 50 %, demonstrating an enhanced role of secondary formation in BrC in recent years. The long-term changes in eBC and BrC have also affected the radiative forcing effect. The direct radiative forcing (Delta F-R) of BC decreased by 67% from +3.36 W m(-2) in 2012 to +1.09 W m(-2) in 2020, and that of BrC decreased from +0.30 to +0.17 W m(-2) during 2018-2020. Such changes might have important implications for affecting aerosol-boundary layer interactions and the improvement of future air quality.
学科领域	Environmental Sciences; Meteorology & Atmospheric Sciences
语种	英语
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号	WOS:000746443600001
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/273533
作者单位	Chinese Academy of Sciences; Institute of Atmospheric Physics, CAS; Chinese Academy of Sciences; University of Chinese Academy of Sciences, CAS; Jinan University; Tianjin University; Chinese Academy of Sciences; Institute of Urban Environment, CAS; Peking University
推荐引用方式 GB/T 7714	Sun, Jiaxing,Wang, Zhe,Zhou, Wei,et al. Measurement report: Long-term changes in black carbon and aerosol optical properties from 2012 to 2020 in Beijing, China[J],2022,22(1):15.
APA	Sun, Jiaxing.,Wang, Zhe.,Zhou, Wei.,Xie, Conghui.,Wu, Cheng.,...&Sun, Yele.(2022).Measurement report: Long-term changes in black carbon and aerosol optical properties from 2012 to 2020 in Beijing, China.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(1),15.
MLA	Sun, Jiaxing,et al."Measurement report: Long-term changes in black carbon and aerosol optical properties from 2012 to 2020 in Beijing, China".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.1(2022):15.