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DOI10.5194/acp-22-10993-2022
Polar stratospheric nitric acid depletion surveyed from a decadal dataset of IASI total columns
Wespes, Catherine; Ronsmans, Gaetane; Clarisse, Lieven; Solomon, Susan; Hurtmans, Daniel; Clerbaux, Cathy; Coheur, Pierre-Francois
发表日期2022
ISSN1680-7316
EISSN1680-7324
起始页码10993
结束页码11007
卷号22期号:16页码:15
英文摘要In this paper, we exploit the first 10-year data record (2008-2017) of nitric acid (HNO3) total columns measured by the IASI-A/MetOp infrared sounder, characterized by an exceptional daily sampling and a good vertical sensitivity in the lower-to-mid stratosphere (around 50 hPa), to monitor the relationship between the temperature decrease and the observed HNO3 loss that occurs each year in the Antarctic stratosphere during the polar night. Since the HNO3 depletion results from the formation of polar stratospheric clouds (PSCs), which trigger the development of the ozone (O3) hole, its continuous monitoring is of high importance. We verify here, from the 10-year time evolution of HNO3 together with temperature (taken from reanalysis at 50 hPa), the recurrence of specific regimes in the annual cycle of IASI HNO3 and identify (for each year) the day and the 50 hPa temperature (drop temperature) corresponding to the onset of strong HNO3 depletion in the Antarctic winter. Although the measured HNO3 total column does not allow for the uptake of HNO3 by different types of PSC particles along the vertical profile to be differentiated, an average drop temperature of 194.2 +/- 3.8 K, close to the nitric acid trihydrate (NAT) existence threshold (similar to 195 K at 50 hPa), is found in the region of potential vorticity lower than -10 x 10-5 Km2kg-1s-1 (similar to the 70-90 circle S equivalent latitude region during winter). The spatial distribution and interannual variability of the drop temperature are investigated and discussed. This paper highlights the capability of the IASI sounder to monitor the evolution of polar stratospheric HNO3, a key player in the processes involved in the depletion of stratospheric O3.
学科领域Environmental Sciences; Meteorology & Atmospheric Sciences
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000847385900001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/273489
作者单位Universite Libre de Bruxelles; Massachusetts Institute of Technology (MIT); Centre National de la Recherche Scientifique (CNRS); UDICE-French Research Universities; Sorbonne Universite; Universite Paris Cite; Universite Paris Saclay
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GB/T 7714
Wespes, Catherine,Ronsmans, Gaetane,Clarisse, Lieven,et al. Polar stratospheric nitric acid depletion surveyed from a decadal dataset of IASI total columns[J],2022,22(16):15.
APA Wespes, Catherine.,Ronsmans, Gaetane.,Clarisse, Lieven.,Solomon, Susan.,Hurtmans, Daniel.,...&Coheur, Pierre-Francois.(2022).Polar stratospheric nitric acid depletion surveyed from a decadal dataset of IASI total columns.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(16),15.
MLA Wespes, Catherine,et al."Polar stratospheric nitric acid depletion surveyed from a decadal dataset of IASI total columns".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.16(2022):15.
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