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DOI | 10.5194/acp-23-3311-2023 |
Global impact of the COVID-19 lockdown on surface concentration and health riskof atmospheric benzene | |
Ling, Chaohao; Cui, Lulu; Li, Rui | |
发表日期 | 2023 |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
起始页码 | 3311 |
结束页码 | 3324 |
卷号 | 23期号:5页码:14 |
英文摘要 | To curb the spread of the COVID-19 pandemic, many countries around the world imposed an unprecedented lockdown, producing reductions in pollutant emissions. Unfortunately, the lockdown-driven global ambient benzene changes still remain unknown. An ensemble machine-learning model coupled with chemical transport models (CTMs) was applied to estimate global high-resolution ambient benzene levels. Afterwards, the extreme gradient boosting (XGBoost) algorithm was employed to decouple the contributions of meteorology and emission reduction to ambient benzene. The change ratio (P-dew) of the deweathered benzene concentration from the pre-lockdown to lockdown period was in the order of India (-23.6 %) > Europe (-21.9 %) > the United States (-16.2 %) > China (-15.6 %). The detrended change (P*) of the deweathered benzene level (change ratio in 2020 - change ratio in 2019) followed the order of India (P*=-16.2 %) > Europe (P*=-13.9 %) > China (P*=-13.3 %) > the United States (P*=-6.00 %). Emission reductions derived from industrial activities and transportation were major drivers for the benzene decrease during the lockdown period. The highest decreasing ratio of ambient benzene in India might be associated with local serious benzene pollution during the business-as-usual period and restricted transportation after lockdown. Substantial decreases in atmospheric benzene levels had significant health benefits. The global average lifetime carcinogenic risk (LCR) and hazard index (HI) decreased from 4.89x10(-7) and 5.90x10(-3 )to 4.51x10(-7) and 5.40x10(-3), respectively. China and India showed higher health benefits due to benzene pollution mitigation compared with other countries, highlighting the importance of benzene emission reduction. |
学科领域 | Environmental Sciences; Meteorology & Atmospheric Sciences |
语种 | 英语 |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000949470900001 |
来源期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/273348 |
作者单位 | MinNan Normal University; Tsinghua University; East China Normal University |
推荐引用方式 GB/T 7714 | Ling, Chaohao,Cui, Lulu,Li, Rui. Global impact of the COVID-19 lockdown on surface concentration and health riskof atmospheric benzene[J],2023,23(5):14. |
APA | Ling, Chaohao,Cui, Lulu,&Li, Rui.(2023).Global impact of the COVID-19 lockdown on surface concentration and health riskof atmospheric benzene.ATMOSPHERIC CHEMISTRY AND PHYSICS,23(5),14. |
MLA | Ling, Chaohao,et al."Global impact of the COVID-19 lockdown on surface concentration and health riskof atmospheric benzene".ATMOSPHERIC CHEMISTRY AND PHYSICS 23.5(2023):14. |
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