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DOI10.5194/acp-23-1091-2023
Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019
Li, Ye; Huang, Ye; Zhang, Yunshan; Du, Wei; Zhang, Shanshan; He, Tianhao; Li, Yan; Chen, Yan; Ding, Fangfang; Huang, Lin; Xia, Haibin; Meng, Wenjun; Liu, Min; Tao, Shu
发表日期2023
ISSN1680-7316
EISSN1680-7324
起始页码1091
结束页码1101
卷号23期号:2页码:11
英文摘要Polychlorinated biphenyls (PCBs) are nowadays mainly unintentionally produced, since their use and manufacture has been banned. PCBs, especially those dioxin-like compounds, have been proven harmful to ecosystems and human health. Detailed information about the spatiotemporally distribution of unintentionally produced PCBs (UP-PCBs) is crucial for understanding the environmental fate and associated health risks. How-ever, research estimating UP-PCBs emission in China is limited. In this study, a source-specific and year-varying emission factor (EF) dataset was used to compile provincial emissions of 12 dioxin-like UP-PCBs congeners for 66 sources in the Chinese mainland from 1960 to 2019. In addition to that, emissions for 2019 were allocated into 0.1 degrees x 0.1 degrees grids. The results indicated that historical national UP-PCBs emission represented an increasing trend until around 1995 and then showed an overall decreasing trend from 1995 to 2019. Cement production was the largest UP-PCBs emission source in the Chinese mainland. Geographically, East and North China con-tributed the largest UP-PCBs emission across the Chinese mainland. High emission densities occurred mainly in the densely populated and well-developed regions such as Yangtze River Delta Urban Agglomeration and Pearl River Delta. Furthermore, highly positive correlations of emission densities with population and GDP densities were identified.
学科领域Environmental Sciences; Meteorology & Atmospheric Sciences
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000921383400001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/273216
作者单位East China Normal University; Peking University; Nanjing Forestry University; Kunming University of Science & Technology
推荐引用方式
GB/T 7714
Li, Ye,Huang, Ye,Zhang, Yunshan,et al. Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019[J],2023,23(2):11.
APA Li, Ye.,Huang, Ye.,Zhang, Yunshan.,Du, Wei.,Zhang, Shanshan.,...&Tao, Shu.(2023).Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019.ATMOSPHERIC CHEMISTRY AND PHYSICS,23(2),11.
MLA Li, Ye,et al."Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019".ATMOSPHERIC CHEMISTRY AND PHYSICS 23.2(2023):11.
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