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DOI | 10.5194/acp-23-1091-2023 |
Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019 | |
Li, Ye; Huang, Ye; Zhang, Yunshan; Du, Wei; Zhang, Shanshan; He, Tianhao; Li, Yan; Chen, Yan; Ding, Fangfang; Huang, Lin; Xia, Haibin; Meng, Wenjun; Liu, Min; Tao, Shu | |
发表日期 | 2023 |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
起始页码 | 1091 |
结束页码 | 1101 |
卷号 | 23期号:2页码:11 |
英文摘要 | Polychlorinated biphenyls (PCBs) are nowadays mainly unintentionally produced, since their use and manufacture has been banned. PCBs, especially those dioxin-like compounds, have been proven harmful to ecosystems and human health. Detailed information about the spatiotemporally distribution of unintentionally produced PCBs (UP-PCBs) is crucial for understanding the environmental fate and associated health risks. How-ever, research estimating UP-PCBs emission in China is limited. In this study, a source-specific and year-varying emission factor (EF) dataset was used to compile provincial emissions of 12 dioxin-like UP-PCBs congeners for 66 sources in the Chinese mainland from 1960 to 2019. In addition to that, emissions for 2019 were allocated into 0.1 degrees x 0.1 degrees grids. The results indicated that historical national UP-PCBs emission represented an increasing trend until around 1995 and then showed an overall decreasing trend from 1995 to 2019. Cement production was the largest UP-PCBs emission source in the Chinese mainland. Geographically, East and North China con-tributed the largest UP-PCBs emission across the Chinese mainland. High emission densities occurred mainly in the densely populated and well-developed regions such as Yangtze River Delta Urban Agglomeration and Pearl River Delta. Furthermore, highly positive correlations of emission densities with population and GDP densities were identified. |
学科领域 | Environmental Sciences; Meteorology & Atmospheric Sciences |
语种 | 英语 |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000921383400001 |
来源期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/273216 |
作者单位 | East China Normal University; Peking University; Nanjing Forestry University; Kunming University of Science & Technology |
推荐引用方式 GB/T 7714 | Li, Ye,Huang, Ye,Zhang, Yunshan,et al. Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019[J],2023,23(2):11. |
APA | Li, Ye.,Huang, Ye.,Zhang, Yunshan.,Du, Wei.,Zhang, Shanshan.,...&Tao, Shu.(2023).Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019.ATMOSPHERIC CHEMISTRY AND PHYSICS,23(2),11. |
MLA | Li, Ye,et al."Temporal and spatial variations in atmospheric unintentional PCB emissionsin Chinese mainland from 1960 to 2019".ATMOSPHERIC CHEMISTRY AND PHYSICS 23.2(2023):11. |
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