气候变化领域集成服务门户(CCPortal): The pathway of impacts of aerosol direct effects on secondary inorganic aerosol formation

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DOI	10.5194/acp-22-5147-2022
	The pathway of impacts of aerosol direct effects on secondary inorganic aerosol formation
	Wang, Jiandong; Xing, Jia; Wang, Shuxiao; Mathur, Rohit; Wang, Jiaping; Zhang, Yuqiang; Liu, Chao; Pleim, Jonathan; Ding, Dian; Chang, Xing; Jiang, Jingkun; Zhao, Peng; Sahu, Shovan Kumar; Jin, Yuzhi; Wong, David C.; Hao, Jiming
发表日期	2022
ISSN	1680-7316
EISSN	1680-7324
起始页码	5147
结束页码	5156
卷号	22 期号:8 页码:10
英文摘要	Airborne aerosols reduce surface solar radiation through light scattering and absorption (aerosol direct effects, ADEs), influence regional meteorology, and further affect atmospheric chemical reactions and aerosol concentrations. The inhibition of turbulence and the strengthened atmospheric stability induced by ADEs increases surface primary aerosol concentration, but the pathway of ADE impacts on secondary aerosol is still unclear. In this study, the online coupled meteorological and chemistry model (WRF-CMAQ; Weather Research and Forecasting-Community Multiscale Air Quality) with integrated process analysis was applied to explore how ADEs affect secondary aerosol formation through changes in atmospheric dynamics and photolysis processes. The meteorological condition and air quality in the Jing-Jin-Ji area (denoted JJJ, including Beijing, Tianjin, and Hebei Province in China) in January and July 2013 were simulated to represent winter and summer conditions, respectively. Our results show that ADEs through the photolysis pathway inhibit sulfate formation during winter in the JJJ region and promote sulfate formation in July. The differences are attributed to the alteration of effective actinic flux affected by single-scattering albedo (SSA). ADEs through the dynamics pathway act as an equally or even more important route compared with the photolysis pathway in affecting secondary aerosol concentration in both summer and winter. ADEs through dynamics traps formed sulfate within the planetary boundary layer (PBL) which increases sulfate concentration in winter. Meanwhile, the impact of ADEs through dynamics is mainly reflected in the increase of gaseous-precursor concentrations within the PBL which enhances secondary aerosol formation in summer. For nitrate, reduced upward transport of precursors restrains the formation at high altitude and eventually lowers the nitrate concentration within the PBL in winter, while such weakened vertical transport of precursors increases nitrate concentration within the PBL in summer, since nitrate is mainly formed near the surface ground.
学科领域	Environmental Sciences; Meteorology & Atmospheric Sciences
语种	英语
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号	WOS:000792368600001
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/273118
作者单位	China Meteorological Administration; Nanjing University of Information Science & Technology; Tsinghua University; United States Environmental Protection Agency; Nanjing University; Duke University; Xi'an Jiaotong-Liverpool University
推荐引用方式 GB/T 7714	Wang, Jiandong,Xing, Jia,Wang, Shuxiao,et al. The pathway of impacts of aerosol direct effects on secondary inorganic aerosol formation[J],2022,22(8):10.
APA	Wang, Jiandong.,Xing, Jia.,Wang, Shuxiao.,Mathur, Rohit.,Wang, Jiaping.,...&Hao, Jiming.(2022).The pathway of impacts of aerosol direct effects on secondary inorganic aerosol formation.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(8),10.
MLA	Wang, Jiandong,et al."The pathway of impacts of aerosol direct effects on secondary inorganic aerosol formation".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.8(2022):10.