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DOI10.5194/acp-23-3325-2023
A high-resolution satellite-based map of global methane emissions reveals missing wetland, fossil fuel, and monsoon sources
Yu, Xueying; Millet, Dylan B.; Henze, Daven K.; Turner, Alexander J.; Delgado, Alba Lorente; Bloom, A. Anthony; Sheng, Jianxiong
发表日期2023
ISSN1680-7316
EISSN1680-7324
起始页码3325
结束页码3346
卷号23期号:5页码:22
英文摘要We interpret space-borne observations from the TROPOspheric Monitoring Instrument (TROPOMI) in a multi-inversion framework to characterize the 2018-2019 global methane budget. Evaluation of the inverse solutions indicates that simultaneous source + sink optimization using methane observations alone remains an ill-posed problem - even with the dense TROPOMI sampling coverage. Employing remote carbon monoxide (CO) and hydroxyl radical (OH) observations with independent methane measurements to distinguish between candidate solutions, we infer from TROPOMI a global methane source of 587 (586-589) Tg yr(-1) and sink of 571 Tg yr(-1) for our analysis period. We apply a new downscaling method to map the derived monthly emissions to 0.1 degrees x 0.1 degrees resolution, using the results to uncover key gaps in the prior methane budget. The TROPOMI data point to an underestimate of tropical wetland emissions (a posteriori increase of +13 % [6 %-25 %] or 20 [7-25] Tg yr(-1)), with adjustments following regional hydrology. Some simple wetland parameterizations represent these patterns as accurately as more sophisticated process-based models. Emissions from fossil fuel activities are strongly underestimated over the Middle East (+5 [2-6] Tg yr(-1) a posteriori increase) and over Venezuela. The TROPOMI observations also reveal many fossil fuel emission hotspots missing from the prior inventory, including over Mexico, Oman, Yemen, Turkmenistan, Iran, Iraq, Libya, and Algeria. Agricultural methane sources are underestimated in India, Brazil, the California Central Valley, and Asia. Overall, anthropogenic sources worldwide are increased by +19 [11-31] Tg yr(-1) over the prior estimate. More than 45 % of this adjustment occurs over India and Southeast Asia during the summer monsoon (+8.5 [3.1-10.7] Tg in July-October), likely due to rainfall-enhanced emissions from rice, manure, and landfills/sewers, which increase during this season along with the natural wetland source.
学科领域Environmental Sciences; Meteorology & Atmospheric Sciences
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000953028200001
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/272972
作者单位University of Minnesota System; Stanford University; University of Colorado System; University of Colorado Boulder; University of Washington; University of Washington Seattle; California Institute of Technology; National Aeronautics & Space Administration (NASA); NASA Jet Propulsion Laboratory (JPL); Massachusetts Institute of Technology (MIT)
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Yu, Xueying,Millet, Dylan B.,Henze, Daven K.,et al. A high-resolution satellite-based map of global methane emissions reveals missing wetland, fossil fuel, and monsoon sources[J],2023,23(5):22.
APA Yu, Xueying.,Millet, Dylan B..,Henze, Daven K..,Turner, Alexander J..,Delgado, Alba Lorente.,...&Sheng, Jianxiong.(2023).A high-resolution satellite-based map of global methane emissions reveals missing wetland, fossil fuel, and monsoon sources.ATMOSPHERIC CHEMISTRY AND PHYSICS,23(5),22.
MLA Yu, Xueying,et al."A high-resolution satellite-based map of global methane emissions reveals missing wetland, fossil fuel, and monsoon sources".ATMOSPHERIC CHEMISTRY AND PHYSICS 23.5(2023):22.
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