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DOI10.1038/s41893-022-00879-8
Carbon-efficient carbon dioxide electrolysers
Ozden, Adnan; Garcia de Arquer, F. Pelayo; Huang, Jianan Erick; Wicks, Joshua; Sisler, Jared; Miao, Rui Kai; O'Brien, Colin P.; Lee, Geonhui; Wang, Xue; Ip, Alexander H.; Sargent, Edward H.; Sinton, David
发表日期2022
ISSN2398-9629
起始页码563
结束页码573
卷号5期号:7页码:11
英文摘要Renewable electricity-powered CO2 electroreduction offers a sustainable route to transform the chemical industry. Here the authors overview four CO2 electrolysis pathways that could be immune from carbonate formation, a major technological barrier. The electroreduction of CO2 (CO2R) is the conversion of CO2 to renewable fuels and feedstocks, a promising technology that could support the transition from fossil to renewable sources in the chemical industry. Today the viability of CO2R technology is limited by carbonate formation via the reaction of reactant CO2 with hydroxides and the energy cost incurred to regenerate the reactant. In this Review, we analyse the literature on four emerging high single pass CO2 conversion approaches: CO2 regeneration from carbonate, CO2R in acidic media, cascade CO2R-COR and CO2R direct from a capture liquid. We analyse each system, describe the challenges associated with each pathway and outline future research directions towards the goal of ensuring that CO2R is viable and thus scalable.
学科领域Green & Sustainable Science & Technology; Environmental Sciences; Environmental Studies
语种英语
WOS研究方向Science & Technology - Other Topics ; Environmental Sciences & Ecology
WOS记录号WOS:000794100000002
来源期刊NATURE SUSTAINABILITY
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/272744
作者单位University of Toronto; Barcelona Institute of Science & Technology; Universitat Politecnica de Catalunya; Institut de Ciencies Fotoniques (ICFO); University of Toronto
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GB/T 7714
Ozden, Adnan,Garcia de Arquer, F. Pelayo,Huang, Jianan Erick,et al. Carbon-efficient carbon dioxide electrolysers[J],2022,5(7):11.
APA Ozden, Adnan.,Garcia de Arquer, F. Pelayo.,Huang, Jianan Erick.,Wicks, Joshua.,Sisler, Jared.,...&Sinton, David.(2022).Carbon-efficient carbon dioxide electrolysers.NATURE SUSTAINABILITY,5(7),11.
MLA Ozden, Adnan,et al."Carbon-efficient carbon dioxide electrolysers".NATURE SUSTAINABILITY 5.7(2022):11.
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