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DOI | 10.1029/2021JD036379 |
Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions | |
Wu, Dianming; Zhang, Jingwei; Wang, Mengdi; An, Junling; Wang, Ruhai; Haider, Haroon; Xu-Ri; Huang, Ye; Zhang, Qiang; Zhou, Feng; Tian, Hanqin; Zhang, Xiuying; Deng, Lingling; Pan, Yuepeng; Chen, Xi; Yu, Yuanchun; Hu, Chunsheng; Wang, Rui; Song, Yaqi; Gao, Zhiwei; Wang, Yue; Hou, Lijun; Liu, Min | |
通讯作者 | Wu, DM ; Liu, M (通讯作者) |
发表日期 | 2022 |
ISSN | 2169-897X |
EISSN | 2169-8996 |
卷号 | 127期号:6 |
英文摘要 | Abiotic and biotic releases of nitrous acid (HONO) from soils contribute substantially to the missing source of tropospheric HONO and hydroxyl radicals (OH). However, global and regional patterns of soil HONO emissions are rarely quantified, and the contributions of such emissions to atmospheric oxidization capacity are unclear. Here, we present that the best estimate of global soil HONO emissions in 2017 was 9.67 with a range of 7.36-11.99 Tg N yr(-1), and cropland soils accounting for similar to 79%. The analyses also indicate that regional soil HONO emissions enhanced ground OH concentrations by 10%-60% and ozone concentrations by 0.5-1.5 ppb in daytime in the ambient area of Shanghai, China. The impact of soil HONO emissions on OH budgets was more significant in rural than urban areas. These findings suggest that the soil HONO emissions, especially from cropland, could quicken photochemical reactions, and aggravate air pollution in rural areas. |
关键词 | NITRIC-OXIDE EMISSIONSAGRICULTURAL FIELDSATMOSPHERIC HONODYNAMIC CHAMBEROZONE FORMATIONNOX EMISSIONSDAYTIME HONORIVER DELTACHINAIMPACTS |
英文关键词 | nitrous acid; hydroxyl radical; ozone; soil nitrogen cycle; air quality |
语种 | 英语 |
WOS研究方向 | Meteorology & Atmospheric Sciences |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000776467500016 |
来源期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES |
来源机构 | 中国科学院青藏高原研究所 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/260779 |
推荐引用方式 GB/T 7714 | Wu, Dianming,Zhang, Jingwei,Wang, Mengdi,et al. Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions[J]. 中国科学院青藏高原研究所,2022,127(6). |
APA | Wu, Dianming.,Zhang, Jingwei.,Wang, Mengdi.,An, Junling.,Wang, Ruhai.,...&Liu, Min.(2022).Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,127(6). |
MLA | Wu, Dianming,et al."Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 127.6(2022). |
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