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DOI10.1029/2021JD036379
Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions
Wu, Dianming; Zhang, Jingwei; Wang, Mengdi; An, Junling; Wang, Ruhai; Haider, Haroon; Xu-Ri; Huang, Ye; Zhang, Qiang; Zhou, Feng; Tian, Hanqin; Zhang, Xiuying; Deng, Lingling; Pan, Yuepeng; Chen, Xi; Yu, Yuanchun; Hu, Chunsheng; Wang, Rui; Song, Yaqi; Gao, Zhiwei; Wang, Yue; Hou, Lijun; Liu, Min
通讯作者Wu, DM ; Liu, M (通讯作者)
发表日期2022
ISSN2169-897X
EISSN2169-8996
卷号127期号:6
英文摘要Abiotic and biotic releases of nitrous acid (HONO) from soils contribute substantially to the missing source of tropospheric HONO and hydroxyl radicals (OH). However, global and regional patterns of soil HONO emissions are rarely quantified, and the contributions of such emissions to atmospheric oxidization capacity are unclear. Here, we present that the best estimate of global soil HONO emissions in 2017 was 9.67 with a range of 7.36-11.99 Tg N yr(-1), and cropland soils accounting for similar to 79%. The analyses also indicate that regional soil HONO emissions enhanced ground OH concentrations by 10%-60% and ozone concentrations by 0.5-1.5 ppb in daytime in the ambient area of Shanghai, China. The impact of soil HONO emissions on OH budgets was more significant in rural than urban areas. These findings suggest that the soil HONO emissions, especially from cropland, could quicken photochemical reactions, and aggravate air pollution in rural areas.
关键词NITRIC-OXIDE EMISSIONSAGRICULTURAL FIELDSATMOSPHERIC HONODYNAMIC CHAMBEROZONE FORMATIONNOX EMISSIONSDAYTIME HONORIVER DELTACHINAIMPACTS
英文关键词nitrous acid; hydroxyl radical; ozone; soil nitrogen cycle; air quality
语种英语
WOS研究方向Meteorology & Atmospheric Sciences
WOS类目Meteorology & Atmospheric Sciences
WOS记录号WOS:000776467500016
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
来源机构中国科学院青藏高原研究所
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/260779
推荐引用方式
GB/T 7714
Wu, Dianming,Zhang, Jingwei,Wang, Mengdi,et al. Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions[J]. 中国科学院青藏高原研究所,2022,127(6).
APA Wu, Dianming.,Zhang, Jingwei.,Wang, Mengdi.,An, Junling.,Wang, Ruhai.,...&Liu, Min.(2022).Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,127(6).
MLA Wu, Dianming,et al."Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 127.6(2022).
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